The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Block Copolymer Templating Syntheses of Mesoporous Metal Oxides with Large Ordering Lengths and Semicrystalline Framework
Abstract
A simple and general procedure has been developed for the syntheses of ordered large-pore (up to 14 nm) mesoporous metal oxides, including TiO 2, ZrO 2, Nb 2 O 5, Ta 2 O 5, Al 2 O 3, SiO 2, SnO 2, WO 3, HfO 2, and mixed oxides SiAlO y, Al 2 TiO y, ZrTiO y, SiTiO y, ZrW 2 O y . Amphiphilic poly(alkylene oxide) block copolymers were used as structure-directing agents in nonaqueous solutions for organizing the network-forming metal oxide species. Inorganic salts, rather than alkoxides or organic metal complexes, were used as soluble and hydrolyzable precursors to the polymerized metal oxide framework. These thermally stable mesoporous oxides have robust inorganic frameworks and thick channel walls, within which high densities of nanocrystallites can be nucleated. These novel mesoporous metal oxides are believed to be formed through a mechanism that combines block copolymer self-assembly with alkylene oxide complexation of the inorganic metal species.
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Citations
Cites
Generalized syntheses of large-pore mesoporous metal oxides with semicrystalline frameworks
Yang, P., Zhao, D., Margolese, D. I., Chmelka, B. F., & Stucky, G. D. (1998) · Nature · doi:10.1038/24132 · Cited by 2,493
Self-citationOrganically modified aluminosilicate mesostructures from block copolymer phases
Templin, M., Franck, A., Du Chesne, A., Leist, H., Zhang, Y., Ulrich, R., Schädler, V., & Wiesner, U. (1997) · Science · doi:10.1126/science.278.5344.1795 · Cited by 668
Cited by
Ordered mesoporous materials in catalysis
Taguchi, A., & Schüth, F. (2005) · Microporous and Mesoporous Materials · doi:10.1016/j.micromeso.2004.06.030 · Cited by 2,119
Nanostructured Tungsten Oxide – Properties, Synthesis, and Applications
Zheng, H., Ou, J. Z., Strano, M. S., Kaner, R. B., Mitchell, A., & Kalantar‐zadeh, K. (2011) · Advanced Functional Materials · doi:10.1002/adfm.201002477 · Cited by 1,479
Characterization of the porous structure of sba-15
Kruk, M., Jaroniec, M., Ko, C. H., & Ryoo, R. (2000) · Chemistry of Materials · doi:10.1021/cm000164e · Cited by 1,409
Synthesis and Characterization of Ion‐Exchangeable Titanate Nanotubes
Sun, X., & Li, Y. (2003) · Chemistry – A European Journal · doi:10.1002/chem.200204394 · Cited by 939
50th Anniversary Perspective: Block Polymers—Pure Potential
Bates, C. M., & Bates, F. S. (2017) · Macromolecules · doi:10.1021/acs.macromol.6b02355 · Cited by 788
Metadata
- Authors
- Yang, P., Zhao, D., Margolese, D. I., Chmelka, B. F., & Stucky, G. D.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 1999-09-29
- Volume
- 11
- Issue
- 10
- Pages
- 2813-2826
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2007524382
- Cited by
- 1,135
- References
- 2
- FWCI
- 28.02
- Type
- journal article
- Language
- en
- Open access
- closed
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