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Tropospheric Halogen Chemistry: Sources, Cycling, and Impacts
Open accessAbstract
In the past 40 years, atmospheric chemists have come to realize that halogens exert a powerful influence on the chemical composition of the troposphere and through that influence affect the fate of pollutants and may affect climate. Of particular note for climate is that halogen cycles affect methane, ozone, and particles, all of which are powerful climate forcing agents through direct and indirect radiative effects. This influencecomes from the high reactivity of atomic halogen radicals (e.g.,Cl, Br, I) and halogen oxides (e.g., ClO, BrO, IO, and higher oxides), known as reactive halogen species in this review. These reactive halogens are potent oxidizers for organic and inorganic compounds throughout the troposphere.
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Cites
Stratospheric sink for chlorofluoromethanes: chlorine atom-catalysed destruction of ozone
Molina, M. J., & Rowland, F. S. (1974) · Nature · doi:10.1038/249810a0 · Cited by 4,332
High levels of nitryl chloride in the polluted subtropical marine boundary layer
Osthoff, H. D., Roberts, J. M., Ravishankara, A. R., Williams, E. J., Lerner, B. M., Sommariva, R., Bates, T. S., Coffman, D., Quinn, P. K., Dibb, J. E., et al. (2008) · Nature Geoscience · doi:10.1038/ngeo177 · Cited by 483
Self-citationHigh winter ozone pollution from carbonyl photolysis in an oil and gas basin
Edwards, P. M., Brown, S. S., Roberts, J. M., Ahmadov, R., Banta, R. M., deGouw, J. A., Dubé, W. P., Field, R. A., Flynn, J. H., Gilman, J. B., et al. (2014) · Nature · doi:10.1038/nature13767 · Cited by 404
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The acidity of atmospheric particles and clouds
Pye, H. O. T., Nenes, A., Alexander, B., Ault, A. P., Barth, M. C., Clegg, S. L., Collett Jr., J. L., Fahey, K. M., Hennigan, C. J., Herrmann, H., et al. (2020) · Atmospheric Chemistry and Physics · doi:10.5194/acp-20-4809-2020 · Cited by 785
Liu, T., Chan, A. W. H., & Abbatt, J. P. D. (2021) · Environmental Science & Technology · doi:10.1021/acs.est.0c06496 · Cited by 292
CHIMERE-2017: from urban to hemispheric chemistry-transport modeling
Mailler, S., Menut, L., Khvorostyanov, D., Valari, M., Couvidat, F., Siour, G., Turquety, S., Briant, R., Tuccella, P., Bessagnet, B., et al. (2017) · Geoscientific Model Development · doi:10.5194/gmd-10-2397-2017 · Cited by 268
Health and Safety Effects of Airborne Soil Dust in the Americas and Beyond
Tong, D. Q., Gill, T. E., Sprigg, W. A., Van Pelt, R. S., Baklanov, A. A., Barker, B. M., Bell, J. E., Castillo, J., Gassó, S., Gaston, C. J., et al. (2023) · Reviews of Geophysics · doi:10.1029/2021rg000763 · Cited by 131
Natural short-lived halogens exert an indirect cooling effect on climate
Saiz-Lopez, A., Fernandez, R. P., Li, Q., Cuevas, C. A., Fu, X., Kinnison, D. E., Tilmes, S., Mahajan, A. S., Gómez Martín, J. C., Iglesias-Suarez, F., et al. (2023) · Nature · doi:10.1038/s41586-023-06119-z · Cited by 91
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Metadata
- Authors
- Simpson, W. R., Brown, S. S., Saiz-Lopez, A., Thornton, J. A., & von Glasow, R.
- Venue
- Chemical Reviews
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-03-12
- Volume
- 115
- Issue
- 10
- Pages
- 4035-4062
- ISSN
- 0009-2665 (ISSN-L)
- 1520-6890
- OpenAlex
- W2019942612
- Cited by
- 556
- References
- 3
- FWCI
- 2.34
- Type
- journal article
- Language
- en
- Open access
- hybrid
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
