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Complete Oxidation of Formaldehyde at Room Temperature Using TiO2 Supported Metallic Pd Nanoparticles
Abstract
A series of reduced and oxidized Pd/TiO 2 catalysts were prepared and used for catalytic oxidation of formaldehyde (HCHO) at room temperature. The reduced catalysts were much more active than the oxidized ones. Nearly 100% HCHO conversion was achieved over the former while it was less than 18% over the latter. Sodium borohydride (NaBH 4 ) reduced Pd/TiO 2 catalysts exhibited very high turnover frequencies of HCHO oxidation and kept highly active in the presence of chloride. Strong metal−support interaction, well-dispersed and negatively charged metallic Pd nanoparticles, and rich chemisorbed oxygen are probably responsible for the high catalytic activities over the former. Metallic Pd nanoparticles with a strong capacity for oxygen activation should be the active sites for catalytic oxidation of HCHO.
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Cites
Identification of Active Gold Nanoclusters on Iron Oxide Supports for CO Oxidation
Herzing, A. A., Kiely, C. J., Carley, A. F., Landon, P., & Hutchings, G. J. (2008) · Science · doi:10.1126/science.1159639 · Cited by 1,530
Cited by
Low temperature catalytic oxidation of volatile organic compounds: a review
Huang, H., Xu, Y., Feng, Q., & Leung, D. Y. C. (2015) · Catalysis Science & Technology · doi:10.1039/c4cy01733a · Cited by 770
Self-citationSurface oxygen vacancies on Co3O4 mediated catalytic formaldehyde oxidation at room temperature
Wang, Z., Wang, W., Zhang, L., & Jiang, D. (2016) · Catalysis Science & Technology · doi:10.1039/c5cy01709b · Cited by 386
Support Morphology-Dependent Catalytic Activity of Pd/CeO2for Formaldehyde Oxidation
Tan, H., Wang, J., Yu, S., & Zhou, K. (2015) · Environmental Science & Technology · doi:10.1021/acs.est.5b01264 · Cited by 371
Hierarchical Core–Shell Al2O3@Pd-CoAlO Microspheres for Low-Temperature Toluene Combustion
Zhao, S., Hu, F., & Li, J. (2016) · ACS Catalysis · doi:10.1021/acscatal.6b00144 · Cited by 355
Wang, X., Peng, X., Ran, H., Lin, B., Ni, J., Lin, J., & Jiang, L. (2018) · Industrial & Engineering Chemistry Research · doi:10.1021/acs.iecr.8b04915 · Cited by 64
Metadata
- Authors
- Huang, H., & Leung, D. Y. C.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-03-03
- Volume
- 1
- Issue
- 4
- Pages
- 348-354
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2030207534
- Cited by
- 308
- References
- 1
- FWCI
- 5.58
- Type
- journal article
- Language
- en
- Open access
- closed
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