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Ceria-Doped Ni/SBA-16 Catalysts for Dry Reforming of Methane
Abstract
Ni-ceria nanoparticles (Ni/Ce = 1/1) in the cage-like pores of SBA-16 were prepared and evaluated in methane dry reforming reactions. Coexistence of ceria in NiCe/SBA-16 resulted in forming uniformly sized Ni particles (av. 5.7 nm) within the mesopores of SBA-16, because of the confinement effect from the framework of SBA-16 and the strong interaction between Ni and ceria. Ceria addition facilitated the reduction of NiCe/SBA-16 compared with Ni/SBA-16, and Ce 3+ was the dominant species in both fresh and used NiCe/SBA-16 catalysts, as determined by Ce L III -edge X-ray absorption near-edge structure (XANES). The methane conversion was much more stable on NiCe/SBA-16 than on Ni/CeO 2 and Ni/SBA-16 in the methane dry reforming at 973 K during a 100 h reaction period; the deactivation of the Ni catalyst and the collapse of the SBA-16 framework were preferably suppressed for NiCe/SBA-16 under the reaction conditions. The remarkable effect of ceria on the structural stability of both the active Ni particles and the SBA-16 framework led to the consistent catalytic performance of NiCe/SBA-16 in methane dry reforming.
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Citations
Cites
Sing, K. S. W. (1985) · Pure and Applied Chemistry · doi:10.1351/pac198557040603 · Cited by 24,485
Cited by
Effect of NiAl2O4 Formation on Ni/Al2O3 Stability during Dry Reforming of Methane
Zhou, L., Li, L., Wei, N., Li, J., & Basset, J. (2015) · ChemCatChem · doi:10.1002/cctc.201500379 · Cited by 276
Metadata
- Authors
- Zhang, S., Muratsugu, S., Ishiguro, N., & Tada, M.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-07-22
- Volume
- 3
- Issue
- 8
- Pages
- 1855-1864
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2324355796
- Cited by
- 347
- References
- 1
- FWCI
- 9.76
- Type
- journal article
- Language
- en
- Open access
- closed
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