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Catalytic Reduction of Biomass-Derived Furanic Compounds with Hydrogen
Abstract
Furfural and 5-hydroxymethylfurfural (HMF) are important platform chemicals in biorefinery. Reduction of furfural or HMF with H 2 over heterogeneous catalysts is the simplest way to convert the oxygen-rich compounds. However, the process can involve many types of reactions such as hydrogenation of the C═O bond, hydrogenation of the furan ring, C–O hydrogenolysis, rearrangement, C–C dissociation, and polymerization. Hydrogenation reactions are most studied in line with hydrogenations of other α,β-unsaturated aldehydes, and it becomes possible to produce each product selectively: furfuryl alcohol, tetrahydrofurfuryl alcohol, 2,5-bis(hydroxymethyl)furan, or 2,5-bis(hydroxymethyl)tetrahydrofuran. Total reduction of side substituents to give 2-methylfuran or 2,5-dimethylfuran is another well-known reaction. Rearrangement and C–O hydrogenolysis reactions have been recently investigated, and they can give useful products such as cyclopentanone, 1,5-pentanediol, and 1,6-hexanediol. Ongoing studies of the reaction mechanisms are also reviewed.
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Cites
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Hydroxymethylfurfural, A Versatile Platform Chemical Made from Renewable Resources
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Furfural—A Promising Platform for Lignocellulosic Biofuels
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Catalytic conversion of biomass to monofunctional hydrocarbons and targeted liquid-fuel classes
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Cited by
Furfural: a renewable and versatile platform molecule for the synthesis of chemicals and fuels
Mariscal, R., Maireles-Torres, P., Ojeda, M., Sádaba, I., & López Granados, M. (2016) · Energy & Environmental Science · doi:10.1039/c5ee02666k · Cited by 1,642
Furfural: A Promising Platform Compound for Sustainable Production of C4 and C5 Chemicals
Li, X., Jia, P., & Wang, T. (2016) · ACS Catalysis · doi:10.1021/acscatal.6b01838 · Cited by 834
Hu, L., Lin, L., Wu, Z., Zhou, S., & Liu, S. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.02.042 · Cited by 445
De, S., Saha, B., & Luque, R. (2015) · Bioresource Technology · doi:10.1016/j.biortech.2014.09.065 · Cited by 359
Bio-Based Chemicals from Renewable Biomass for Integrated Biorefineries
Kohli, K., Prajapati, R., & Sharma, B. K. (2019) · Energies · doi:10.3390/en12020233 · Cited by 357
Metadata
- Authors
- Nakagawa, Y., Tamura, M., & Tomishige, K.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-10-24
- Volume
- 3
- Issue
- 12
- Pages
- 2655-2668
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2317704676
- Cited by
- 701
- References
- 6
- FWCI
- 23.91
- Type
- journal article
- Language
- en
- Open access
- closed
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