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Vanadium-Node-Functionalized UiO-66: A Thermally Stable MOF-Supported Catalyst for the Gas-Phase Oxidative Dehydrogenation of Cyclohexene
Abstract
The OH groups on the Zr-based nodes of ultrastable UiO-66 can be metallated with V V ions in a facile fashion to give the derivative VUiO-66. This metallated MOF exhibits high stability over a broad temperature range and displays high selectivity for benzene under low-conversion conditions in the vapor-phase oxidative dehydrogenation of cyclohexene (activation energy ∼110 kJ/mol). The integrity of the MOF is maintained after catalysis as determined by PXRD, ICP-AES, and SEM.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Self-citationHorike, S., Shimomura, S., & Kitagawa, S. (2009) · Nature Chemistry · doi:10.1038/nchem.444 · Cited by 2,486
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Zhu, X., Li, B., Yang, J., Li, Y., Zhao, W., Shi, J., & Gu, J. (2015) · ACS Applied Materials & Interfaces · doi:10.1021/am5059074 · Cited by 486
Metal-organic frameworks: Challenges and opportunities for ion-exchange/sorption applications
Kumar, P., Pournara, A., Kim, K.-H., Bansal, V., Rapti, S., & Manos, M. J. (2017) · Progress in Materials Science · doi:10.1016/j.pmatsci.2017.01.002 · Cited by 423
When defects turn into virtues: The curious case of zirconium-based metal-organic frameworks
Taddei, M. (2017) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.04.010 · Cited by 341
Engineering UiO‐66 Metal Organic Framework for Heterogeneous Catalysis
Dhakshinamoorthy, A., Santiago‐Portillo, A., Asiri, A. M., & Garcia, H. (2019) · ChemCatChem · doi:10.1002/cctc.201801452 · Cited by 298
Metadata
- Authors
- Nguyen, H. G. T., Schweitzer, N. M., Chang, C.-Y., Drake, T. L., So, M. C., Stair, P. C., Farha, O. K., Hupp, J. T., & Nguyen, S. T.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-06-30
- Volume
- 4
- Issue
- 8
- Pages
- 2496-2500
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2075804376
- Cited by
- 231
- References
- 2
- FWCI
- 8.03
- Type
- journal article
- Language
- en
- Open access
- closed
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