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Potential Remediation of Waters Contaminated with Cr(III), Cu, and Zn by Sorption on the Organic Polymeric Fraction of Olive Mill Wastewater (Polymerin) and Its Derivatives
Abstract
A study on the individual sorption of Cr(III), Cu, and Zn on polymerin, the humic-acid-like fraction of olive mill wastewater, and its derivatives, K-polymerin and an Fe(OH)x-polymerin complex, showed that these heavy metals were strongly sorbed on polymerin and K-polymerin in the order Cr(III) > Cu > Zn. The sorption on Fe(OH)x-polymerin was to a lower extent compared with that of the other two sorbents, but to a higher extent compared with ferrihydride [Fe(OH)x]. Combined atomic absorption spectrometry and diffuse reflectance infrared Fourier transform spectroscopy analyses showed that the selected heavy metals were individually sorbed on polymerin by means of a cation exchange mechanism, which was consistent with the replacement of Ca, Mg, K, and H bound to the carboxylate groups of the biosorbent and the concomitant chelation of the heavy metals by the OH groups of polymerin polysaccharide component. In binary combination and equimolar ratio, Cu was sorbed by polymerin more selectively than Zn. In ternary combination and equimolar ratio, Cr(III), Cu, and Zn were sorbed by polymerin in the order Cr(III) > Cu > Zn. The sorbing capacity of Zn and Cu was strongly influenced by Cr(III), whereas the sorbing capacity of Cr(III) was not affected bythe presence of the other two metals. The overall sorbing capacity of the binary and ternary mixtures of the three metals on polymerin proved to be considerable and much greater than that on Fe(OH)x-polymerin. Simulated wastewaters cont…
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In the presence of equimolar Zn concentrations, the sorbed Cu amounts were only slightly reduced when compared with the amounts sorbed in the absence of Zn.
“In the presence of equimolar Zn concentrations, the sorbed Cu amounts were only slightly reduced when compared with the amounts sorbed in the absence of Zn.”
From MOBILITY AND BIOAVAILABILITY OF HEAVY METALS AND METALLOIDS IN SOIL ENVIRONMENTS (2010) · cites this paper as Capasso et al., 2004
On POL as well as on ferrihydrite, Cu was sorbed more selectively than Zn.
“On POL as well as on ferrihydrite, Cu was sorbed more selectively than Zn.”
From MOBILITY AND BIOAVAILABILITY OF HEAVY METALS AND METALLOIDS IN SOIL ENVIRONMENTS (2010) · cites this paper as Capasso et al., 2004
Conversely, the Cu presence strongly reduced Zn sorption.
“Conversely, the Cu presence strongly reduced Zn sorption.”
From MOBILITY AND BIOAVAILABILITY OF HEAVY METALS AND METALLOIDS IN SOIL ENVIRONMENTS (2010) · cites this paper as Capasso et al., 2004
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Metadata
- Authors
- Capasso, R., Pigna, M., De Martino, A., Pucci, M., Sannino, F., & Violante, A.
- Affiliations
- University of Naples Federico II (IT)
- Dipartimento di Scienze del Suolo della Pianta e dell'Ambiente, Università degli Studi di Napoli “Federico II”, 80055 Portici (NA), Italy
- Corresponding author
- Capasso, Renato
- ORCID
- Sannino, Filomena
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-08-27
- Volume
- 38
- Issue
- 19
- Pages
- 5170-5176
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2063489085
- Cited by
- 35
- References
- 19
- Citations by year
- 2023: 1 · 2020: 1 · 2018: 2 · 2013: 3 · 2012: 2
- FWCI
- 4.09
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Environmental Science & Technology (publishedVersion)
- PubMed (publishedVersion)
- Funders
- Università degli Studi di Napoli Federico II
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
- Physical Sciences › Environmental Science › Water Science and Technology › Heavy Metal Pollution Remediation
- Physical Sciences › Environmental Science › Water Science and Technology › Coagulation and Flocculation Studies
- Keywords
- heavy metal adsorption, olive mill wastewater, trivalent chromium, copper, zinc, biosorption, cation exchange, carboxylate groups, ferrihydrite, sorption capacity, wastewater remediation, adsorbent regeneration
- MeSH terms
- Adsorption, Biodegradation, Environmental, Chromium, Copper, Industrial Waste, Polymers, Waste Disposal, Fluid, Zinc, Water Purification, Olea
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