The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Particle Phase Acidity and Oligomer Formation in Secondary Organic Aerosol
Open accessAbstract
A series of controlled laboratory experiments are carried out in dual Teflon chambers to examine the presence of oligomers in secondary organic aerosols (SOA) from hydrocarbon ozonolysis as well as to explore the effect of particle phase acidity on SOA formation. In all seven hydrocarbon systems studied (i.e., alpha-pinene, cyclohexene, 1-methyl cyclopentene, cycloheptene, 1-methyl cyclohexene, cyclooctene, and terpinolene), oligomers with MW from 250 to 1600 are present in the SOA formed, both in the absence and presence of seed particles and regardless of the seed particle acidity. These oligomers are comparable to, and in some cases, exceed the low molecular weight species (MW < 250) in ion intensities in the ion trap mass spectra, suggesting they may comprise a substantial fraction of the total aerosol mass. It is possible that oligomers are widely present in atmospheric organic aerosols, formed through acid- or base-catalyzed heterogeneous reactions. In addition, as the seed particle acidity increases, larger oligomers are formed more abundantly in the SOA; consequently, the overall SOA yield also increases. This explicit effect of particle phase acidity on the composition and yield of SOA may have important climatic consequences and need to be considered in relevant models.
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Cites
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Macpherson, A. J., & Uhr, T. (2004) · Science · doi:10.1126/science.1091334 · Cited by 1,584
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Self-citationHeterogeneous Atmospheric Aerosol Production by Acid-Catalyzed Particle-Phase Reactions
Jang, M., Czoschke, N. M., Lee, S., & Kamens, R. M. (2002) · Science · doi:10.1126/science.1075798 · Cited by 1,034
Identification of Polymers as Major Components of Atmospheric Organic Aerosols
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Organic Atmospheric Particulate Material
Seinfeld, J. H., & Pankow, J. F. (2003) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.54.011002.103756 · Cited by 561
Self-citationFormation of Oligomers in Secondary Organic Aerosol
Tolocka, M. P., Jang, M., Ginter, J. M., Cox, F. J., Kamens, R. M., & Johnston, M. V. (2004) · Environmental Science & Technology · doi:10.1021/es035030r · Cited by 506
Robotic Observations of Dust Storm Enhancement of Carbon Biomass in the North Pacific
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Self-citationOrganosulfate Formation in Biogenic Secondary Organic Aerosol
Surratt, J. D., Gómez-González, Y., Chan, A. W. H., Vermeylen, R., Shahgholi, M., Kleindienst, T. E., Edney, E. O., Offenberg, J. H., Lewandowski, M., Jaoui, M., et al. (2008) · The Journal of Physical Chemistry A · doi:10.1021/jp802310p · Cited by 730
Self-citationThe effect of physical and chemical aerosol properties on warm cloud droplet activation
McFiggans, G., Artaxo, P., Baltensperger, U., Coe, H., Facchini, M. C., Feingold, G., Fuzzi, S., Gysel, M., Laaksonen, A., Lohmann, U., et al. (2006) · Atmospheric Chemistry and Physics · doi:10.5194/acp-6-2593-2006 · Cited by 710
The Molecular Identification of Organic Compounds in the Atmosphere: State of the Art and Challenges
Nozière, B., Kalberer, M., Claeys, M., Allan, J., D’Anna, B., Decesari, S., Finessi, E., Glasius, M., Grgić, I., Hamilton, J. F., et al. (2015) · Chemical Reviews · doi:10.1021/cr5003485 · Cited by 656
Aqueous chemistry and its role in secondary organic aerosol (SOA) formation
Lim, Y. B., Tan, Y., Perri, M. J., Seitzinger, S. P., & Turpin, B. J. (2010) · Atmospheric Chemistry and Physics · doi:10.5194/acp-10-10521-2010 · Cited by 585
Metadata
- Authors
- Gao, S., Ng, N. L., Keywood, M., Varutbangkul, V., Bahreini, R., Nenes, A., He, J., Yoo, K. Y., Beauchamp, J. L., Hodyss, R. P., Flagan, R. C., & Seinfeld, J. H.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-11-12
- Volume
- 38
- Issue
- 24
- Pages
- 6582-6589
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2133032938
- Cited by
- 353
- References
- 10
- FWCI
- 16.54
- Type
- journal article
- Language
- en
- Open access
- green
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