The DOI matches its Crossref record; 53 of the 53 references it cites were found in a registry or an index.
Epoxide Pathways Improve Model Predictions of Isoprene Markers and Reveal Key Role of Acidity in Aerosol Formation
Abstract
Isoprene significantly contributes to organic aerosol in the southeastern United States where biogenic hydrocarbons mix with anthropogenic emissions. In this work, the Community Multiscale Air Quality model is updated to predict isoprene aerosol from epoxides produced under both high- and low-NOx conditions. The new aqueous aerosol pathways allow for explicit predictions of two key isoprene-derived species, 2-methyltetrols and 2-methylglyceric acid, that are more consistent with observations than estimates based on semivolatile partitioning. The new mechanism represents a significant source of organic carbon in the lower 2 km of the atmosphere and captures the abundance of 2-methyltetrols relative to organosulfates during the simulation period. For the parametrization considered here, a 25% reduction in SOx emissions effectively reduces isoprene aerosol, while a similar reduction in NOx leads to small increases in isoprene aerosol.
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Cites
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Reactive intermediates revealed in secondary organic aerosol formation from isoprene
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Self-citationA review of Secondary Organic Aerosol (SOA) formation from isoprene
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Unexpected Epoxide Formation in the Gas-Phase Photooxidation of Isoprene
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Secondary Organic Aerosol Formation from Isoprene Photooxidation
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The acidity of atmospheric particles and clouds
Pye, H. O. T., Nenes, A., Alexander, B., Ault, A. P., Barth, M. C., Clegg, S. L., Collett Jr., J. L., Fahey, K. M., Hennigan, C. J., Herrmann, H., et al. (2020) · Atmospheric Chemistry and Physics · doi:10.5194/acp-20-4809-2020 · Cited by 785
Self-citationCompilation of Henry's law constants (version 5.0.0) for water as solvent
Sander, R. (2023) · Atmospheric Chemistry and Physics · doi:10.5194/acp-23-10901-2023 · Cited by 474
Appel, K. W., Bash, J. O., Fahey, K. M., Foley, K. M., Gilliam, R. C., Hogrefe, C., Hutzell, W. T., Kang, D., Mathur, R., Murphy, B. N., et al. (2021) · Geoscientific Model Development · doi:10.5194/gmd-14-2867-2021 · Cited by 408
Self-citationMarais, E. A., Jacob, D. J., Jimenez, J. L., Campuzano-Jost, P., Day, D. A., Hu, W., Krechmer, J., Zhu, L., Kim, P. S., Miller, C. C., et al. (2016) · Atmospheric Chemistry and Physics · doi:10.5194/acp-16-1603-2016 · Cited by 342
Self-citationAppel, K. W., Napelenok, S. L., Foley, K. M., Pye, H. O. T., Hogrefe, C., Luecken, D. J., Bash, J. O., Roselle, S. J., Pleim, J. E., Foroutan, H., et al. (2017) · Geoscientific Model Development · doi:10.5194/gmd-10-1703-2017 · Cited by 336
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Metadata
- Authors
- Pye, H. O. T., Pinder, R. W., Piletic, I. R., Xie, Y., Capps, S. L., Lin, Y.-H., Surratt, J. D., Zhang, Z., Gold, A., Luecken, D. J., Hutzell, W. T., Jaoui, M., Offenberg, J. H., Kleindienst, T. E., Lewandowski, M., & Edney, E. O.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-09-11
- Volume
- 47
- Issue
- 19
- Pages
- 11056-11064
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W1987244498
- Cited by
- 280
- References
- 53
- FWCI
- 13.20
- Type
- journal article
- Language
- en
- Open access
- closed
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- Pye, H. O. T., Pinder, R. W., Piletic, I. R., Xie, Y., Capps, S. L., Lin, Y.-H., Surratt, J. D., Zhang, Z., Gold, A., Luecken, D. J., Hutzell, W. T., Jaoui, M., Offenberg, J. H., Kleindienst, T. E., Lewandowski, M., & Edney, E. O. (2013). Epoxide Pathways Improve Model Predictions of Isoprene Markers and Reveal Key Role of Acidity in Aerosol Formation. Environmental Science & Technology. https://doi.org/10.1021/es402106h
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
