The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Secondary organic aerosol formation from anthropogenic air pollution: Rapid and higher than expected
Open accessAbstract
The atmospheric chemistry of volatile organic compounds (VOCs) in urban areas results in the formation of ‘photochemical smog’, including secondary organic aerosol (SOA). State‐of‐the‐art SOA models parameterize the results of simulation chamber experiments that bracket the conditions found in the polluted urban atmosphere. Here we show that in the real urban atmosphere reactive anthropogenic VOCs (AVOCs) produce much larger amounts of SOA than these models predict, even shortly after sunrise. Contrary to current belief, a significant fraction of the excess SOA is formed from first‐generation AVOC oxidation products. Global models deem AVOCs a very minor contributor to SOA compared to biogenic VOCs (BVOCs). If our results are extrapolated to other urban areas, AVOCs could be responsible for additional 3–25 Tg yr−1 SOA production globally, and cause up to −0.1 W m−2 additional top‐of‐the‐atmosphere radiative cooling.
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Cites
Aerosols, Climate, and the Hydrological Cycle
Ramanathan, V., Crutzen, P. J., Kiehl, J. T., & Rosenfeld, D. (2001) · Science · doi:10.1126/science.1064034 · Cited by 3,831
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Evolution of Organic Aerosols in the Atmosphere
Jimenez, J. L., Canagaratna, M. R., Donahue, N. M., Prevot, A. S. H., Zhang, Q., Kroll, J. H., DeCarlo, P. F., Allan, J. D., Coe, H., Ng, N. L., et al. (2009) · Science · doi:10.1126/science.1180353 · Cited by 4,167
Self-citationFormation of Urban Fine Particulate Matter
Zhang, R., Wang, G., Guo, S., Zamora, M. L., Ying, Q., Lin, Y., Wang, W., Hu, M., & Wang, Y. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00067 · Cited by 1,426
Volatile chemical products emerging as largest petrochemical source of urban organic emissions
McDonald, B. C., de Gouw, J. A., Gilman, J. B., Jathar, S. H., Akherati, A., Cappa, C. D., Jimenez, J. L., Lee-Taylor, J., Hayes, P. L., McKeen, S. A., et al. (2018) · Science · doi:10.1126/science.aaq0524 · Cited by 1,373
Self-citationA review of biomass burning: Emissions and impacts on air quality, health and climate in China
Chen, J., Li, C., Ristovski, Z., Milic, A., Gu, Y., Islam, M. S., Wang, S., Hao, J., Zhang, H., He, C., et al. (2017) · Science of The Total Environment · doi:10.1016/j.scitotenv.2016.11.025 · Cited by 1,262
Reactive intermediates revealed in secondary organic aerosol formation from isoprene
Surratt, J. D., Chan, A. W. H., Eddingsaas, N. C., Chan, M., Loza, C. L., Kwan, A. J., Hersey, S. P., Flagan, R. C., Wennberg, P. O., & Seinfeld, J. H. (2010) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0911114107 · Cited by 1,081
Metadata
- Authors
- Volkamer, R., Jimenez, J. L., San Martini, F., Dzepina, K., Zhang, Q., Salcedo, D., Molina, L. T., Worsnop, D. R., & Molina, M. J.
- Venue
- Geophysical Research Letters
- Publisher
- American Geophysical Union (AGU)
- Published
- 2006-09
- Volume
- 33
- Issue
- 17
- ISSN
- 0094-8276 (ISSN-L)
- 1944-8007
- OpenAlex
- W2052859509
- Cited by
- 1,153
- References
- 1
- FWCI
- 43.58
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Volkamer, R., Jimenez, J. L., San Martini, F., Dzepina, K., Zhang, Q., Salcedo, D., Molina, L. T., Worsnop, D. R., & Molina, M. J. (2006). Secondary organic aerosol formation from anthropogenic air pollution: Rapid and higher than expected. Geophysical Research Letters. https://doi.org/10.1029/2006gl026899
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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