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Synthesis of Sintering-Resistant Sorbents for CO2 Capture
Abstract
Sorbents for high temperature CO2 capture are under intensive development owing to their potential applications in advanced zero emission power, sorption-enhanced steam methane reforming for hydrogen production and energy storage systems in chemical heat pumps. One of the challenges in the development is the prevention of sintering of the sorbent (normally a calcium oxide derivative) which causes the CO2 capture capacity of the material to deteriorate rapidly after a few cycles of utilization. Here we show that a simple wet mixing method can produce sintering-resistant sorbents from calcium and magnesium salts of d-gluconic acid. It was found that calcium oxide was well distributed in the sorbents with metal oxide nanoparticles on the surface acting as physical barriers, and the CO2 capture capacity of the sorbents was largely maintained over multiple cycles of utilization. This method was also applied to other organometallic salts of calcium and magnesium/aluminum and the produced sorbents showed similarly high reversibility.
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Cites
Lackner, K. S. (2003) · Science · doi:10.1126/science.1079033 · Cited by 1,290
Cited by
Synthesis of micro and nano-sized calcium carbonate particles and their applications
Boyjoo, Y., Pareek, V. K., & Liu, J. (2014) · J. Mater. Chem. A · doi:10.1039/c4ta02070g · Cited by 421
Dean, C. C., Blamey, J., Florin, N. H., Al-Jeboori, M. J., & Fennell, P. S. (2011) · Chemical Engineering Research and Design · doi:10.1016/j.cherd.2010.10.013 · Cited by 375
Calcium looping sorbents for CO2 capture
Erans, M., Manovic, V., & Anthony, E. J. (2016) · Applied Energy · doi:10.1016/j.apenergy.2016.07.074 · Cited by 369
Performance Enhancement of Calcium Oxide Sorbents for Cyclic CO2 Capture—A Review
Liu, W., An, H., Qin, C., Yin, J., Wang, G., Feng, B., & Xu, M. (2012) · Energy & Fuels · doi:10.1021/ef300220x · Cited by 320
Self-citationHigh temperature capture of CO2 on lithium-based sorbents from rice husk ash
Wang, K., Guo, X., Zhao, P., Wang, F., & Zheng, C. (2011) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2011.02.040 · Cited by 130
Metadata
- Authors
- Liu, W., Feng, B., Wu, Y., Wang, G., Barry, J., & Diniz da Costa, J. C.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-03-05
- Volume
- 44
- Issue
- 8
- Pages
- 3093-3097
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2016490797
- Cited by
- 239
- References
- 1
- FWCI
- 31.03
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, W., Feng, B., Wu, Y., Wang, G., Barry, J., & Diniz da Costa, J. C. (2010). Synthesis of Sintering-Resistant Sorbents for CO2 Capture. Environmental Science & Technology. https://doi.org/10.1021/es903436v
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