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Nitrate-Induced Photolysis in Natural Waters: Controls on Concentrations of Hydroxyl Radical Photo-Intermediates by Natural Scavenging Agents
Abstract
The importance of the principal natural scavenging agents for hydroxyl radicals ( • OH) was evaluated, and a general framework was developed to predict the significance of nitrate-induced, • OH-mediated degradation of aquatic contaminants. Rate constants for • OH scavenging by dissolved organic matter (DOM) from five surface water sources were in a narrow range (2.3 ± 0.77 × 10 4 (mg of C/L) - 1 s - 1 ), which is similar to previously reported values and suggests that the importance of DOM as a • OH sink can be estimated simply from the dissolved organic carbon (DOC) concentration of a water. Scavenging of • OH by carbonate and bicarbonate is generally less important, but these ions can be the major cause of • OH scavenging in low DOC, high alkalinity waters. Use of the framework is illustrated by predicting levels of • OH and half-lives of the corn herbicide acetochlor in waters ranging from pristine to highly influenced by agricultural activities.
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Metadata
- Authors
- Brezonik, P. L., & Fulkerson-Brekken, J.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 1998-08-26
- Volume
- 32
- Issue
- 19
- Pages
- 3004-3010
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W1980448791
- Cited by
- 480
- References
- 1
- FWCI
- 7.62
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
