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Poly(allylamine)–Mesoporous Silica Composite Materials for CO2 Capture from Simulated Flue Gas or Ambient Air
Abstract
Low-molecular-weight poly(allylamine) is prepared via free-radical polymerization, and the resulting polymer is impregnated into mesocellular silica foams at different amine loadings. The resulting poly(allylamine)–silica composites are demonstrated as effective adsorbents for the extraction of carbon dioxide from dilute (simulated flue gas) and ultradilute (simulated ambient air) gas streams. The composite adsorbents are shown to have comparable adsorption capacities to more-conventional poly(ethyleneimine)–silica adsorbents. Potential advantages of poly(allylamine)-derived adsorbents are discussed.
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Citations
Cited by
Direct Capture of CO2 from Ambient Air
Sanz-Pérez, E. S., Murdock, C. R., Didas, S. A., & Jones, C. W. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00173 · Cited by 2,406
Self-citationAir as the renewable carbon source of the future: an overview of CO2 capture from the atmosphere
Goeppert, A., Czaun, M., Surya Prakash, G. K., & Olah, G. A. (2012) · Energy & Environmental Science · doi:10.1039/c2ee21586a · Cited by 724
Sorbents for the Direct Capture of CO 2 from Ambient Air
Shi, X., Xiao, H., Azarabadi, H., Song, J., Wu, X., Chen, X., & Lackner, K. S. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201906756 · Cited by 679
CO2-Induced Degradation of Amine-Containing Adsorbents: Reaction Products and Pathways
Sayari, A., Heydari-Gorji, A., & Yang, Y. (2012) · Journal of the American Chemical Society · doi:10.1021/ja304888a · Cited by 365
CO2 capture adsorbents functionalized by amine – bearing polymers: A review
Varghese, A. M., & Karanikolos, G. N. (2020) · International Journal of Greenhouse Gas Control · doi:10.1016/j.ijggc.2020.103005 · Cited by 363
Metadata
- Authors
- Chaikittisilp, W., Khunsupat, R., Chen, T. T., & Jones, C. W.
- Venue
- Industrial & Engineering Chemistry Research
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-11-29
- Volume
- 50
- Issue
- 24
- Pages
- 14203-14210
- ISSN
- 0888-5885 (ISSN-L)
- 1520-5045
- OpenAlex
- W2011661984
- Cited by
- 222
- References
- 0
- FWCI
- 24.47
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chaikittisilp, W., Khunsupat, R., Chen, T. T., & Jones, C. W. (2011). Poly(allylamine)–Mesoporous Silica Composite Materials for CO2 Capture from Simulated Flue Gas or Ambient Air. Industrial & Engineering Chemistry Research. https://doi.org/10.1021/ie201584t
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