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Adsorption and Diffusion of Carbon Dioxide on Metal−Organic Framework (MOF-5)
Abstract
Adsorption equilibrium and diffusion of CO 2 on microporous metal−organic frameworks (MOF-5, or IRMOF-1) crystals were experimentally studied by the gravimetric method in the pressure range up to 1 atm. The MOF-5 crystal cubes of about 40−60 μm in sizes were synthesized by the solvothermal method. Freundlich adsorption isotherm equation can fit well CO 2 adsorption isotherms on MOF-5, with isosteric heat of adsorption of about 34 kJ/mol. Diffusion coefficient of CO 2 in the MOF-5 is in the range of 8.1−11.5 × 10 −9 cm 2 /s in 295−331K with activation energy of 7.61 kJ/mol. MOF-5 offers attractive adsorption properties as an adsorbent for separation of CO 2 from flue gas.
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Citations
Cited by
Metal–Organic Frameworks for Separations
Li, J.-R., Sculley, J., & Zhou, H.-C. (2012) · Chemical Reviews · doi:10.1021/cr200190s · Cited by 6,323
Carbon Dioxide Capture: Prospects for New Materials
D'Alessandro, D. M., Smit, B., & Long, J. R. (2010) · Angewandte Chemie International Edition · doi:10.1002/anie.201000431 · Cited by 4,046
CO2 capture by solid adsorbents and their applications: current status and new trends
Wang, Q., Luo, J., Zhong, Z., & Borgna, A. (2011) · Energy Environ. Sci. · doi:10.1039/c0ee00064g · Cited by 1,611
Sinha, A., Darunte, L. A., Jones, C. W., Realff, M. J., & Kawajiri, Y. (2017) · Industrial & Engineering Chemistry Research · doi:10.1021/acs.iecr.6b03887 · Cited by 282
Sorbents for CO2 capture from flue gas—aspects from materials and theoretical chemistry
Hedin, N., Chen, L., & Laaksonen, A. (2010) · Nanoscale · doi:10.1039/c0nr00042f · Cited by 243
Metadata
- Authors
- Zhao, Z., Li, Z., & Lin, Y. S.
- Venue
- Industrial & Engineering Chemistry Research
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-11-18
- Volume
- 48
- Issue
- 22
- Pages
- 10015-10020
- ISSN
- 0888-5885 (ISSN-L)
- 1520-5045
- OpenAlex
- W2095204227
- Cited by
- 347
- References
- 0
- FWCI
- 9.99
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhao, Z., Li, Z., & Lin, Y. S. (2009). Adsorption and Diffusion of Carbon Dioxide on Metal−Organic Framework (MOF-5). Industrial & Engineering Chemistry Research. https://doi.org/10.1021/ie900665f
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