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Carbon Dioxide Hydrogenation To Form Methanol via a Reverse-Water-Gas-Shift Reaction (the CAMERE Process)
Abstract
The CAMERE process (carbon dioxide hydrogenation to form methanol via a reverse-water-gas-shift reaction) was developed and evaluated. The reverse-water-gas-shift reactor and the methanol synthesis reactor were serially aligned to form methanol from CO 2 hydrogenation. Carbon dioxide was converted to CO and water by the reverse-water-gas-shift reaction (RWReaction) to remove water before methanol was synthesized. With the elimination of water by RWReaction, the purge gas volume was minimized as the recycle gas volume decreased. Because of the minimum purge gas loss by the pretreatment of RWReactor, the overall methanol yield increased up to 89% from 69%. An active and stable catalyst with the composition of Cu/ZnO/ZrO 2 /Ga 2 O 3 (5:3:1:1) was developed. The system was optimized and compared with the commercial methanol synthesis processes from natural gas and coal.
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Citations
Cited by
Klankermayer, J., Wesselbaum, S., Beydoun, K., & Leitner, W. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201507458 · Cited by 856
A Review of The Methanol Economy: The Fuel Cell Route
Simon Araya, S., Liso, V., Cui, X., Li, N., Zhu, J., Sahlin, S. L., Jensen, S. H., Nielsen, M. P., & Kær, S. K. (2020) · Energies · doi:10.3390/en13030596 · Cited by 298
Study of iron-promoted Cu/SiO2 catalyst on high temperature reverse water gas shift reaction
Chen, C.-S., Cheng, W.-H., & Lin, S.-S. (2004) · Applied Catalysis A: General · doi:10.1016/s0926-860x(03)00637-9 · Cited by 265
Kim, J., Henao, C. A., Johnson, T. A., Dedrick, D. E., Miller, J. E., Stechel, E. B., & Maravelias, C. T. (2011) · Energy & Environmental Science · doi:10.1039/c1ee01311d · Cited by 262
Life cycle assessment of CO 2 -based C1-chemicals
Sternberg, A., Jens, C. M., & Bardow, A. (2017) · Green Chemistry · doi:10.1039/c6gc02852g · Cited by 212
Metadata
- Authors
- Joo, O.-S., Jung, K.-D., Moon, I., Rozovskii, A. Y., Lin, G. I., Han, S.-H., & Uhm, S.-J.
- Venue
- Industrial & Engineering Chemistry Research
- Publisher
- American Chemical Society (ACS)
- Published
- 1999-04-01
- Volume
- 38
- Issue
- 5
- Pages
- 1808-1812
- ISSN
- 0888-5885 (ISSN-L)
- 1520-5045
- OpenAlex
- W1969108284
- Cited by
- 322
- References
- 0
- FWCI
- 1.07
- Type
- journal article
- Language
- en
- Open access
- closed
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- Joo, O.-S., Jung, K.-D., Moon, I., Rozovskii, A. Y., Lin, G. I., Han, S.-H., & Uhm, S.-J. (1999). Carbon Dioxide Hydrogenation To Form Methanol via a Reverse-Water-Gas-Shift Reaction (the CAMERE Process). Industrial & Engineering Chemistry Research. https://doi.org/10.1021/ie9806848
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
