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Multistimuli, Multiresponsive Metallo-Supramolecular Polymers
Abstract
The use of metal ion-induced polymerizations of a ditopic ligand offers a facile route to the preparation of organic/inorganic hybrid materials. Such metallo-supramolecular polymers potentially offer the functionality of the metal ion along with the processibility of a polymer. We report, herein, the preparation of gellike metallo-supramolecular polymers prepared from a monomer unit, which consists of a 2,6-bis-(benzimidazolyl)-4-hydroxypyridine unit attached to either end of a polyether chain, mixed with a transition metal ion (e.g., Co(II) or Zn(II)) and a small percentage of a lanthanoid metal (e.g., La(III), Eu(III)). Such materials show dramatic reversible responses to a variety of stimuli, including thermal, mechanical, chemo, and photo. The nature of the response can be controlled by the nature of the combination of transition metal ion and lanthanide metal ion used.
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Citations
Cited by
Yan, X., Xu, D., Chi, X., Chen, J., Dong, S., Ding, X., Yu, Y., & Huang, F. (2012) · Advanced Materials · doi:10.1002/adma.201103220 · Cited by 697
Hydrogen-bonded Supramolecular π-Functional Materials
González-Rodríguez, D., & Schenning, A. P. H. J. (2011) · Chemistry of Materials · doi:10.1021/cm101817h · Cited by 426
Two‐Component Gel‐Phase Materials—Highly Tunable Self‐Assembling Systems
Hirst, A. R., & Smith, D. K. (2005) · Chemistry – A European Journal · doi:10.1002/chem.200500241 · Cited by 369
Metadata
- Authors
- Beck, J. B., & Rowan, S. J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2003-10-25
- Volume
- 125
- Issue
- 46
- Pages
- 13922-13923
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2036037731
- Cited by
- 693
- References
- 0
- FWCI
- 11.04
- Type
- journal article
- Language
- en
- Open access
- closed
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