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Influence of Water on the Surface of Hydrophilic and Hydrophobic Room-Temperature Ionic Liquids
Abstract
Vibrational spectroscopy, sum frequency generation, has been used to study the gas-liquid interface of imidazolium-based, room-temperature ionic liquids. The ionic liquids are divided into two categories on the basis of their miscibility with water, as hydrophobic (immiscible) and hydrophilic (miscible). The spectroscopy results indicate that water will reorient the cations of the hydrophobic ionic liquid, while in the hydrophilic ones they remain unaffected. Thus, under low water conditions the plane of the imidazolium ring remains parallel to the surface for both types of ionic liquid. However, at high water content the ring will reorient to along the surface normal for the hydrophobic ionic liquid but remain parallel to the surface for the hydrophilic one. This is a reversible process.
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Cites
Influence of chloride, water, and organic solvents on the physical properties of ionic liquids
Seddon, K. R., Stark, A., & Torres, M.-J. (2000) · Pure and Applied Chemistry · doi:10.1351/pac200072122275 · Cited by 2,293
Cammarata, L., Kazarian, S. G., Salter, P. A., & Welton, T. (2001) · Physical Chemistry Chemical Physics · doi:10.1039/b106900d · Cited by 1,441
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Sun, X., Luo, H., & Dai, S. (2012) · Chemical Reviews · doi:10.1021/cr200193x · Cited by 852
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Jiang, W., Wang, Y., & Voth, G. A. (2007) · The Journal of Physical Chemistry B · doi:10.1021/jp067142l · Cited by 458
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Marcinkowska, R., Konieczna, K., Marcinkowski, Ł., Namieśnik, J., & Kloskowski, A. (2019) · TrAC Trends in Analytical Chemistry · doi:10.1016/j.trac.2019.07.025 · Cited by 119
Metadata
- Authors
- Rivera-Rubero, S., & Baldelli, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-09-01
- Volume
- 126
- Issue
- 38
- Pages
- 11788-11789
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1977854765
- Cited by
- 229
- References
- 2
- FWCI
- 5.73
- Type
- journal article
- Language
- en
- Open access
- closed
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