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Liquid Hydrogen in Protonic Chabazite
Abstract
Due to its fully reversible nature, H(2) storage by molecular adsorption could represent an advantage with respect to dissociative processes, where kinetic effects during the charging and discharging processes are present. A drawback of this strategy is represented by the extremely weak interactions that require low temperature and high pressure. High surface area materials hosting polarizing sites can represent a viable way toward more favorable working conditions. Of these, in this contribution, we have studied hydrogen adsorption in a series of zeolites using volumetric techniques and infrared spectroscopy at 15 K. We have found that in H-SSZ-13 zeolite the cooperative role played by high surface area, internal wall topology, and presence of high binding energy sites (protons) allows hydrogen to densify inside the nanopores at favorable temperature and pressure conditions.
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Cited by
Deep Eutectic Solvents (DESs) and Their Applications
Smith, E. L., Abbott, A. P., & Ryder, K. S. (2014) · Chemical Reviews · doi:10.1021/cr300162p · Cited by 7,378
McKeown, N. B., & Budd, P. M. (2006) · Chemical Society Reviews · doi:10.1039/b600349d · Cited by 1,747
Gas Storage in Nanoporous Materials
Morris, R. E., & Wheatley, P. S. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200703934 · Cited by 1,622
Enhanced Hydrogen Storage Capacity of High Surface Area Zeolite-like Carbon Materials
Yang, Z., Xia, Y., & Mokaya, R. (2007) · Journal of the American Chemical Society · doi:10.1021/ja067149g · Cited by 622
Metal-organic frameworks: structure, properties, methods of synthesis and characterization
Butova, V. V., Soldatov, M. A., Guda, A. A., Lomachenko, K. A., & Lamberti, C. (2016) · Russian Chemical Reviews · doi:10.1070/rcr4554 · Cited by 527
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Metadata
- Authors
- Zecchina, A., Bordiga, S., Vitillo, J. G., Ricchiardi, G., Lamberti, C., Spoto, G., Bjørgen, M., & Lillerud, K. P.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-04-12
- Volume
- 127
- Issue
- 17
- Pages
- 6361-6366
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1970529594
- Cited by
- 215
- References
- 0
- FWCI
- 23.40
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zecchina, A., Bordiga, S., Vitillo, J. G., Ricchiardi, G., Lamberti, C., Spoto, G., Bjørgen, M., & Lillerud, K. P. (2005). Liquid Hydrogen in Protonic Chabazite. Journal of the American Chemical Society. https://doi.org/10.1021/ja050276c
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