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Inorganic Oxide Core, Polymer Shell Nanocomposite as a High K Gate Dielectric for Flexible Electronics Applications
Abstract
Organic/inorganic core shell nanoparticles have been synthesized using high K TiO(2) as the core nanoparticle, and polystyrene as the shell. This material is easy to process and forms transparent continuous thin films, which exhibit a dielectric constant enhancement of over 3 times that of bulk polystyrene. This new dielectric material has been incorporated into capacitors and thin film transistors (TFTs). Mobilities approaching 0.2 cm(2)/V.s have been measured for pentacene TFTs incorporating the new TiO(2) polystyrene nanostructured gate dielectric, indicating good surface properties for pentacene film growth. This novel strategy for generating high K flexible gate dielectrics will be of value in improving organic and flexible electronic device performance.
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Cited by
Barbey, R., Lavanant, L., Paripovic, D., Schüwer, N., Sugnaux, C., Tugulu, S., & Klok, H.-A. (2009) · Chemical Reviews · doi:10.1021/cr900045a · Cited by 1,753
Yang, J. C., Mun, J., Kwon, S. Y., Park, S., Bao, Z., & Park, S. (2019) · Advanced Materials · doi:10.1002/adma.201904765 · Cited by 1,641
Flexible Nanodielectric Materials with High Permittivity for Power Energy Storage
Dang, Z., Yuan, J., Yao, S., & Liao, R. (2013) · Advanced Materials · doi:10.1002/adma.201301752 · Cited by 1,454
Polymers for flexible displays: From material selection to device applications
Choi, M.-C., Kim, Y., & Ha, C.-S. (2008) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2007.11.004 · Cited by 981
High-k Organic, Inorganic, and Hybrid Dielectrics for Low-Voltage Organic Field-Effect Transistors
Ortiz, R. P., Facchetti, A., & Marks, T. J. (2010) · Chemical Reviews · doi:10.1021/cr9001275 · Cited by 871
Li, G. L., Möhwald, H., & Shchukin, D. G. (2013) · Chemical Society Reviews · doi:10.1039/c3cs35517a · Cited by 314
Metadata
- Authors
- Maliakal, A., Katz, H., Cotts, P. M., Subramoney, S., & Mirau, P.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-09-30
- Volume
- 127
- Issue
- 42
- Pages
- 14655-14662
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1999127784
- Cited by
- 225
- References
- 0
- FWCI
- 6.67
- Type
- journal article
- Language
- en
- Open access
- closed
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