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Versatile Precursors of Functional RAFT Agents. Application to the Synthesis of Bio-Related End-Functionalized Polymers
Abstract
Biomolecule-polymer conjugates are widely used in bio-related fields, but their synthesis is often tricky, especially the introduction of a single biomolecule at one chain end. This paper describes a new straightforward approach to prepare such conjugates via RAFT polymerization. By designing appropriate bio-related RAFT agents, polymer chains of controlled chain length (Mn = 10 000-40 000 and PDI < 1.1) carrying a single biomolecule as an alpha-end group (a sugar or a biotin) linked by a stable amide bond are obtained. Considering the versatility of the RAFT process, this strategy appears to be very attractive for the design of a variety of conjugates.
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Citations
Cited by
Radical addition–fragmentation chemistry in polymer synthesis
Moad, G., Rizzardo, E., & Thang, S. H. (2008) · Polymer · doi:10.1016/j.polymer.2007.11.020 · Cited by 1,397
Well-Defined Protein−Polymer Conjugates via in Situ RAFT Polymerization
Boyer, C., Bulmus, V., Liu, J., Davis, T. P., Stenzel, M. H., & Barner-Kowollik, C. (2007) · Journal of the American Chemical Society · doi:10.1021/ja070956a · Cited by 411
Metadata
- Authors
- Bathfield, M., D'Agosto, F., Spitz, R., Charreyre, M.-T., & Delair, T.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-02-02
- Volume
- 128
- Issue
- 8
- Pages
- 2546-2547
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2018948332
- Cited by
- 180
- References
- 0
- FWCI
- 12.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Versatile Precursors of Functional RAFT Agents. Application to the Synthesis of Bio-Related End-Functionalized Polymers. https://app.cochat.ai/papers/10.1021/ja057481c
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- Bathfield, M., D'Agosto, F., Spitz, R., Charreyre, M.-T., & Delair, T. (2006). Versatile Precursors of Functional RAFT Agents. Application to the Synthesis of Bio-Related End-Functionalized Polymers. Journal of the American Chemical Society. https://doi.org/10.1021/ja057481c
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
