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Contrast Viscosity Changes upon Photoirradiation for Mixtures of Poly(acrylic acid)-Based α-Cyclodextrin and Azobenzene Polymers
Abstract
Polymer-polymer interactions were investigated for mixtures of a poly(acrylic acid) (pAA) carrying azobenzene (pC12Azo) and two kinds of pAA carrying alpha-cyclodextrin (CD), in which CDs are attached to the main chain through the 3- and 6-positions in CD (p3alphaCD and p6alphaCD, respectively), using several techniques, such as viscosity and NMR measurements. Viscosity data exhibited contrast changes upon UV irradiation: thinning (p3alphaCD/pC12Azo) and thickening (p6alphaCD/pC12Azo). NOESY spectra confirmed that the contrast viscosity changes were ascribable to differences in how CD moieties interact with pC12Azo after photoisomerization of azobenzene moieties from trans to cis: dissociation of inclusion complexes (p3alphaCD/pC12Azo) and formation of interlocked complexes (p6alphaCD/pC12Azo).
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Introduction and General Overview of Cyclodextrin Chemistry
Szejtli, J. (1998) · Chemical Reviews · doi:10.1021/cr970022c · Cited by 5,016
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Yu, G., Zhou, X., Zhang, Z., Han, C., Mao, Z., Gao, C., & Huang, F. (2012) · Journal of the American Chemical Society · doi:10.1021/ja3099905 · Cited by 486
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Metadata
- Authors
- Tomatsu, I., Hashidzume, A., & Harada, A.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-02-01
- Volume
- 128
- Issue
- 7
- Pages
- 2226-2227
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2021697388
- Cited by
- 242
- References
- 1
- FWCI
- 8.97
- Type
- journal article
- Language
- en
- Open access
- closed
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