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Redox Control within Single-Site Polymerization Catalysts
Abstract
The activity of a single-site titanium-based lactide polymerization initiator supported by a ferrocenyl-derivatized salen ligand is shown to be modulated by a chemical redox switch; a substantially higher rate of propagation is found for the neutral catalyst compared to its oxidized dicationic ferrocenium counterpart.
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Citations
Cited by
Electrochemically Mediated Atom Transfer Radical Polymerization
Magenau, A. J. D., Strandwitz, N. C., Gennaro, A., & Matyjaszewski, K. (2011) · Science · doi:10.1126/science.1202357 · Cited by 804
Biocompatible Initiators for Lactide Polymerization
Platel, R., Hodgson, L., & Williams, C. (2008) · Polymer Reviews · doi:10.1080/15583720701834166 · Cited by 706
Wang, X., Thevenon, A., Brosmer, J. L., Yu, I., Khan, S. I., Mehrkhodavandi, P., & Diaconescu, P. L. (2014) · Journal of the American Chemical Society · doi:10.1021/ja505883u · Cited by 263
Chemoselective Polymerizations from Mixtures of Epoxide, Lactone, Anhydride, and Carbon Dioxide
Romain, C., Zhu, Y., Dingwall, P., Paul, S., Rzepa, H. S., Buchard, A., & Williams, C. K. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.5b13070 · Cited by 258
Guillaume, S. M., Kirillov, E., Sarazin, Y., & Carpentier, J. (2015) · Chemistry – A European Journal · doi:10.1002/chem.201500613 · Cited by 251
Metadata
- Authors
- Gregson, C. K. A., Gibson, V. C., Long, N. J., Marshall, E. L., Oxford, P. J., & White, A. J. P.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-05-19
- Volume
- 128
- Issue
- 23
- Pages
- 7410-7411
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2029653132
- Cited by
- 291
- References
- 0
- FWCI
- 4.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Gregson, C. K. A., Gibson, V. C., Long, N. J., Marshall, E. L., Oxford, P. J., & White, A. J. P. (2006). Redox Control within Single-Site Polymerization Catalysts. Journal of the American Chemical Society. https://doi.org/10.1021/ja061398n
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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