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Hydrogen Storage in Metal−Organic Frameworks by Bridged Hydrogen Spillover
Abstract
The possible utilization of hydrogen as the energy source for fuel-cell vehicles is limited by the lack of a viable hydrogen storage system. Metal-organic frameworks (MOFs) belong to a new class of microporous materials that have recently been shown to be potential candidates for hydrogen storage; however, no significant hydrogen storage capacity has been achieved in MOFs at ambient temperature. Here we report substantially increased hydrogen storage capacities of modified MOFs by using a simple technique that causes and facilitates hydrogen spillover. Thus, the storage of 4 wt % is achieved at room temperature and 100 atm for the modified IRMOF-8. The adsorption is reversible, and the rates are fast. That has made MOFs truly promising for hydrogen storage application.
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Cites
Materials for hydrogen storage
Züttel, A. (2003) · Materials Today · doi:10.1016/s1369-7021(03)00922-2 · Cited by 2,216
Cited by
Defect‐Engineered Metal–Organic Frameworks
Fang, Z., Bueken, B., De Vos, D. E., & Fischer, R. A. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201411540 · Cited by 1,252
Han, S. S., Mendoza-Cortés, J. L., & Goddard III, W. A. (2009) · Chemical Society Reviews · doi:10.1039/b802430h · Cited by 594
Nanoporous Polymers for Hydrogen Storage
Germain, J., Fréchet, J. M. J., & Svec, F. (2009) · Small · doi:10.1002/smll.200801762 · Cited by 432
Recent Progress Using Solid-State Materials for Hydrogen Storage: A Short Review
Lee, S.-Y., Lee, J.-H., Kim, Y.-H., Kim, J.-W., Lee, K.-J., & Park, S.-J. (2022) · Processes · doi:10.3390/pr10020304 · Cited by 229
Metadata
- Authors
- Li, Y., & Yang, R. T.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-06-01
- Volume
- 128
- Issue
- 25
- Pages
- 8136-8137
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2063471264
- Cited by
- 526
- References
- 1
- FWCI
- 28.36
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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