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Defect-Site Promoted Surface Reorganization in Nanocrystalline Ceria for the Low-Temperature Activation of Ethylbenzene
Abstract
Defect-site enriched nanocrystalline ceria prepared by an alcoholysis method favors oxidative dehydrogenation of ethylbenzene using nitrous oxide with high conversion and selectivity at much lower temperatures compared to ceria samples prepared by other conventional methods. A direct correlation exists between the concentration of −Ce 4+ −O - −Ce 3+ -type defect sites and the reaction rates and, hence, the activation temperature required for the reaction.
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Cited by
Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Zheng, A., Liu, S.-B., & Deng, F. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00289 · Cited by 365
Hegde, M. S., Madras, G., & Patil, K. C. (2009) · Accounts of Chemical Research · doi:10.1021/ar800209s · Cited by 337
Wang, Y., Wang, F., Song, Q., Xin, Q., Xu, S., & Xu, J. (2013) · Journal of the American Chemical Society · doi:10.1021/ja310498c · Cited by 324
Highly defective CeO 2 as a promoter for efficient and stable water oxidation
Liang, F., Yu, Y., Zhou, W., Xu, X., & Zhu, Z. (2015) · Journal of Materials Chemistry A · doi:10.1039/c4ta05770h · Cited by 266
Metadata
- Authors
- Murugan, B., & Ramaswamy, A. V.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-02-23
- Volume
- 129
- Issue
- 11
- Pages
- 3062-3063
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2000827309
- Cited by
- 172
- References
- 0
- FWCI
- 3.66
- Type
- journal article
- Language
- en
- Open access
- closed
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- Murugan, B., & Ramaswamy, A. V. (2007). Defect-Site Promoted Surface Reorganization in Nanocrystalline Ceria for the Low-Temperature Activation of Ethylbenzene. Journal of the American Chemical Society. https://doi.org/10.1021/ja066834k
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