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Size-Dependent Electron Injection from Excited CdSe Quantum Dots into TiO2 Nanoparticles
Abstract
Electron injection from excited CdSe quantum dots into TiO 2 nanoparticles can be easily modulated by controlling the particle size. Femtosecond transient absorption studies indicate that the rate constant for electron transfer from the thermalized s-state of CdSe quantum dots increases with decreasing particle size. The energy difference between the conduction bands of the two semiconductor systems acts as a driving force for the electron transfer in the normal Marcus region. An increase in the interparticle electron transfer rate constant by 3 orders of magnitude (from ∼10 7 to 10 10 s -1 ) has been achieved by decreasing the CdSe particle diameter from 7.5 to 2.4 nm.
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Cites
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Self-citationCharacterization of nanostructured hybrid and organic solar cells by impedance spectroscopy
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Dang, X., Yi, H., Ham, M.-H., Qi, J., Yun, D. S., Ladewski, R., Strano, M. S., Hammond, P. T., & Belcher, A. M. (2011) · Nature Nanotechnology · doi:10.1038/nnano.2011.50 · Cited by 396
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Metadata
- Authors
- Robel, I., Kuno, M., & Kamat, P. V.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-03-21
- Volume
- 129
- Issue
- 14
- Pages
- 4136-4137
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2033018647
- Cited by
- 839
- References
- 1
- FWCI
- 26.97
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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