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A High-Mobility Electron-Transport Polymer with Broad Absorption and Its Use in Field-Effect Transistors and All-Polymer Solar Cells
Abstract
An electron-transport polymer with good solution processibility, excellent thermal stability, and high electron affinity based on alternating perylene diimide and dithienothiophene units has been synthesized. Electron mobilities as high as 1.3 × 10 -2 cm 2 V -1 s -1 have been measured in field-effect transistor geometry. The polymer shows broad absorptions throughout the visible and extending into the near-IR. A power conversion efficiency of over 1%, under simulated AM 1.5, 100 mW/cm 2, was measured for a single-layer solar cell using this polymer as an acceptor and a polythiophene derivative as a donor.
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Citations
Cites
Conjugated Polymer-Based Organic Solar Cells
Günes, S., Neugebauer, H., & Sariciftci, N. S. (2007) · Chemical Reviews · doi:10.1021/cr050149z · Cited by 6,279
Cited by
Fused Nonacyclic Electron Acceptors for Efficient Polymer Solar Cells
Dai, S., Zhao, F., Zhang, Q., Lau, T.-K., Li, T., Liu, K., Ling, Q., Wang, C., Lu, X., You, W., et al. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.6b12755 · Cited by 864
Self-citationDesigning π-conjugated polymers for organic electronics
Guo, X., Baumgarten, M., & Müllen, K. (2013) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2013.09.005 · Cited by 836
Single‐Junction Binary‐Blend Nonfullerene Polymer Solar Cells with 12.1% Efficiency
Zhao, F., Dai, S., Wu, Y., Zhang, Q., Wang, J., Jiang, L., Ling, Q., Wei, Z., Ma, W., You, W., et al. (2017) · Advanced Materials · doi:10.1002/adma.201700144 · Cited by 699
Self-citationPolymer donor–polymer acceptor (all-polymer) solar cells
Facchetti, A. (2013) · Materials Today · doi:10.1016/j.mattod.2013.04.005 · Cited by 688
Quinn, J. T. E., Zhu, J., Li, X., Wang, J., & Li, Y. (2017) · Journal of Materials Chemistry C · doi:10.1039/c7tc01680h · Cited by 452
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Metadata
- Authors
- Zhan, X., Tan, Z., Domercq, B., An, Z., Zhang, X., Barlow, S., Li, Y., Zhu, D., Kippelen, B., & Marder, S. R.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-05-18
- Volume
- 129
- Issue
- 23
- Pages
- 7246-7247
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2018094686
- Cited by
- 1,172
- References
- 1
- FWCI
- 50.40
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhan, X., Tan, Z., Domercq, B., An, Z., Zhang, X., Barlow, S., Li, Y., Zhu, D., Kippelen, B., & Marder, S. R. (2007). A High-Mobility Electron-Transport Polymer with Broad Absorption and Its Use in Field-Effect Transistors and All-Polymer Solar Cells. Journal of the American Chemical Society. https://doi.org/10.1021/ja071760d
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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