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A Facile Procedure for Controlling Monomer Sequence Distribution in Radical Chain Polymerizations
Abstract
A novel sequential copolymerization strategy was investigated for preparing macromolecules with programmed sequences of functional comonomers. Four different N -substituted maleimides ( N -propyl maleimide, N -benzyl maleimide, N -methyl maleimide, and N -[3,5-bis(trifluoromethyl)phenyl] maleimide) were consecutively added during the atom transfer radical polymerization of styrene performed at 110 °C in the presence of a catalyst composed of copper(I) bromide and 4,4‘-dinonyl)-2,2‘-bipyridine. Owing to the exceptional cross-propagation of N -substituted maleimides with styrene, the four functional comonomers could be sequentially incorporated in the growing polymer chains.
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Primer-Directed Enzymatic Amplification of DNA with a Thermostable DNA Polymerase
Saiki, R. K., Gelfand, D. H., Stoffel, S., Scharf, S. J., Higuchi, R., Horn, G. T., Mullis, K. B., & Erlich, H. A. (1988) · Science · doi:10.1126/science.2448875 · Cited by 17,719
Macromolecular architectures by living and controlled/living polymerizations
Hadjichristidis, N., Iatrou, H., Pitsikalis, M., & Mays, J. (2006) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2006.07.002 · Cited by 642
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Lutz, J.-F., Ouchi, M., Liu, D. R., & Sawamoto, M. (2013) · Science · doi:10.1126/science.1238149 · Cited by 1,381
Self-citationOuchi, M., Terashima, T., & Sawamoto, M. (2009) · Chemical Reviews · doi:10.1021/cr900234b · Cited by 1,257
Lutz, J. (2008) · Journal of Polymer Science Part A: Polymer Chemistry · doi:10.1002/pola.22706 · Cited by 1,245
Self-citationCorrigan, N., Jung, K., Moad, G., Hawker, C. J., Matyjaszewski, K., & Boyer, C. (2020) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2020.101311 · Cited by 981
Single-chain technology using discrete synthetic macromolecules
Ouchi, M., Badi, N., Lutz, J.-F., & Sawamoto, M. (2011) · Nature Chemistry · doi:10.1038/nchem.1175 · Cited by 386
Self-citationIterative exponential growth of stereo- and sequence-controlled polymers
Barnes, J. C., Ehrlich, D. J. C., Gao, A. X., Leibfarth, F. A., Jiang, Y., Zhou, E., Jamison, T. F., & Johnson, J. A. (2015) · Nature Chemistry · doi:10.1038/nchem.2346 · Cited by 361
Soeriyadi, A. H., Boyer, C., Nyström, F., Zetterlund, P. B., & Whittaker, M. R. (2011) · Journal of the American Chemical Society · doi:10.1021/ja205080u · Cited by 326
Gutekunst, W. R., & Hawker, C. J. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b04940 · Cited by 283
Schmidt, B. V. K. J., Fechler, N., Falkenhagen, J., & Lutz, J.-F. (2011) · Nature Chemistry · doi:10.1038/nchem.964 · Cited by 268
Self-citationKramer, J. W., Treitler, D. S., Dunn, E. W., Castro, P. M., Roisnel, T., Thomas, C. M., & Coates, G. W. (2009) · Journal of the American Chemical Society · doi:10.1021/ja9075327 · Cited by 261
Encoding information into polymers
Rutten, M. G. T. A., Vaandrager, F. W., Elemans, J. A. A. W., & Nolte, R. J. M. (2018) · Nature Reviews Chemistry · doi:10.1038/s41570-018-0051-5 · Cited by 216
The limits of precision monomer placement in chain growth polymerization
Gody, G., Zetterlund, P. B., Perrier, S., & Harrisson, S. (2016) · Nature Communications · doi:10.1038/ncomms10514 · Cited by 170
Metadata
- Authors
- Pfeifer, S., & Lutz, J.-F.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-07-17
- Volume
- 129
- Issue
- 31
- Pages
- 9542-9543
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2084326111
- Cited by
- 319
- References
- 2
- FWCI
- 4.11
- Type
- journal article
- Language
- en
- Open access
- closed
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