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Metal−Organic Polyhedral Frameworks: High H2 Adsorption Capacities and Neutron Powder Diffraction Studies
Abstract
Neutron powder diffraction experiments on D(2)-loaded NOTT-112 reveal that the axial sites of exposed Cu(II) ions in the smallest cuboctahedral cages are the first, strongest binding sites for D(2) leading to an overall discrimination between the two types of exposed Cu(II) sites at the paddlewheel nodes. Thus, the Cu(II) centers within the cuboctahedral cage are the first sites of D(2) binding with a Cu-D(2) distance of 2.23(1) A.
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Citations
Cited by
The Chemistry and Applications of Metal-Organic Frameworks
Furukawa, H., Cordova, K. E., O’Keeffe, M., & Yaghi, O. M. (2013) · Science · doi:10.1126/science.1230444 · Cited by 16,945
Farha, O. K., Özgür Yazaydın, A., Eryazici, I., Malliakas, C. D., Hauser, B. G., Kanatzidis, M. G., Nguyen, S. T., Snurr, R. Q., & Hupp, J. T. (2010) · Nature Chemistry · doi:10.1038/nchem.834 · Cited by 1,741
Li, M., Li, D., O’Keeffe, M., & Yaghi, O. M. (2014) · Chemical Reviews · doi:10.1021/cr400392k · Cited by 1,161
Mesoporous metal–organic framework materials
Xuan, W., Zhu, C., Liu, Y., & Cui, Y. (2012) · Chem. Soc. Rev. · doi:10.1039/c1cs15196g · Cited by 933
Kökçam-Demir, Ü., Goldman, A., Esrafili, L., Gharib, M., Morsali, A., Weingart, O., & Janiak, C. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00609e · Cited by 895
Metadata
- Authors
- Yan, Y., Telepeni, I., Yang, S., Lin, X., Kockelmann, W., Dailly, A., Blake, A. J., Lewis, W., Walker, G. S., Allan, D. R., Barnett, S. A., Champness, N. R., & Schröder, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-03-03
- Volume
- 132
- Issue
- 12
- Pages
- 4092-4094
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2072587093
- Cited by
- 291
- References
- 0
- FWCI
- 25.24
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yan, Y., Telepeni, I., Yang, S., Lin, X., Kockelmann, W., Dailly, A., Blake, A. J., Lewis, W., Walker, G. S., Allan, D. R., Barnett, S. A., Champness, N. R., & Schröder, M. (2010). Metal−Organic Polyhedral Frameworks: High H2 Adsorption Capacities and Neutron Powder Diffraction Studies. Journal of the American Chemical Society. https://doi.org/10.1021/ja1001407
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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