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Direct Electrodeposition of Tetrahexahedral Pd Nanocrystals with High-Index Facets and High Catalytic Activity for Ethanol Electrooxidation
Abstract
Tetrahexahedral Pd nanocrystals (THH Pd NCs) with {730} high-index facets were directly produced on a glassy carbon substrate in a dilute PdCl(2) solution by a newly developed programmed electrodeposition method. The THH Pd NCs, thanks to their high density of surface atomic steps, exhibit 4-6 times higher catalytic activity than commercial Pd black catalyst toward ethanol electrooxidation in alkaline solutions. This straightforward method provides a promising route to facile preparation of high-index-faceted metal nanocatalysts with high catalytic activity.
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Citations
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Tian, N., Zhou, Z.-Y., Sun, S.-G., Ding, Y., & Wang, Z. L. (2007) · Science · doi:10.1126/science.1140484 · Cited by 3,073
Self-citationMechanism of catalysis of hydrocarbon reactions by platinum surfaces
Somorjai, G. A., & Blakely, D. W. (1975) · Nature · doi:10.1038/258580a0 · Cited by 357
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Sub-nanometre sized metal clusters: from synthetic challenges to the unique property discoveries
Lu, Y., & Chen, W. (2012) · Chemical Society Reviews · doi:10.1039/c2cs15325d · Cited by 1,152
High-Index Faceted Noble Metal Nanocrystals
Quan, Z., Wang, Y., & Fang, J. (2013) · Accounts of Chemical Research · doi:10.1021/ar200293n · Cited by 582
Lu, C.-L., Prasad, K. S., Wu, H.-L., Ho, J.-A. A., & Huang, M. H. (2010) · Journal of the American Chemical Society · doi:10.1021/ja105401p · Cited by 389
Shape-controlled syntheses of rhodium nanocrystals for the enhancement of their catalytic properties
Xie, S., Liu, X. Y., & Xia, Y. (2015) · Nano Research · doi:10.1007/s12274-014-0674-x · Cited by 104
Metadata
- Authors
- Tian, N., Zhou, Z.-Y., Yu, N.-F., Wang, L.-Y., & Sun, S.-G.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-05-14
- Volume
- 132
- Issue
- 22
- Pages
- 7580-7581
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1964847069
- Cited by
- 478
- References
- 2
- FWCI
- 22.24
- Type
- journal article
- Language
- en
- Open access
- closed
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- Tian, N., Zhou, Z.-Y., Yu, N.-F., Wang, L.-Y., & Sun, S.-G. (2010). Direct Electrodeposition of Tetrahexahedral Pd Nanocrystals with High-Index Facets and High Catalytic Activity for Ethanol Electrooxidation. Journal of the American Chemical Society. https://doi.org/10.1021/ja102177r
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
