The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Energy Transfer Dynamics in Metal−Organic Frameworks
Abstract
Isomorphous metal-organic frameworks (MOFs) based on {M[4,4'-(HO(2)C)(2)-bpy](2)bpy}(2+) building blocks (where M = Ru or Os) were designed and synthesized to study the classic Ru to Os energy transfer process that has potential applications in light-harvesting with supramolecular assemblies. The crystalline nature of the MOFs allows precise determination of the distances between metal centers by X-ray diffraction, thereby facilitating the study of the Ru→Os energy transfer process. The mixed-metal MOFs with 0.3, 0.6, 1.4, and 2.6 mol % Os doping were also synthesized in order to study the energy transfer dynamics with a two-photon excitation at 850 nm. The Ru lifetime at 620 nm decreases from 171 ns in the pure Ru MOF to 29 ns in the sample with 2.6 mol % Os doping. In the mixed-metal samples, energy transfer was observed with an initial growth in Os emission corresponding with the rate of decay of the Ru excited state. These results demonstrate rapid, efficient energy migration and long distance transfer in isomorphous MOFs.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Cited by
Nanoscale Metal–Organic Frameworks for Biomedical Imaging and Drug Delivery
Della Rocca, J., Liu, D., & Lin, W. (2011) · Accounts of Chemical Research · doi:10.1021/ar200028a · Cited by 2,087
Self-citationA facile synthesis of UiO-66, UiO-67 and their derivatives
Katz, M. J., Brown, Z. J., Colón, Y. J., Siu, P. W., Scheidt, K. A., Snurr, R. Q., Hupp, J. T., & Farha, O. K. (2013) · Chemical Communications · doi:10.1039/c3cc46105j · Cited by 1,756
Metal–Organic Frameworks for Light Harvesting and Photocatalysis
Wang, J.-L., Wang, C., & Lin, W. (2012) · ACS Catalysis · doi:10.1021/cs3005874 · Cited by 802
Self-citationHigh-throughput computational screening of metal–organic frameworks
Colón, Y. J., & Snurr, R. Q. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00070f · Cited by 470
Pore Chemistry of Metal–Organic Frameworks
Ji, Z., Wang, H., Canossa, S., Wuttke, S., & Yaghi, O. M. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202000238 · Cited by 459
Metadata
- Authors
- Kent, C. A., Mehl, B. P., Ma, L., Papanikolas, J. M., Meyer, T. J., & Lin, W.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-08-25
- Volume
- 132
- Issue
- 37
- Pages
- 12767-12769
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1969324795
- Cited by
- 355
- References
- 1
- FWCI
- 13.20
- Type
- journal article
- Language
- en
- Open access
- closed
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