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An Efficient Nickel Catalyst for the Reduction of Carbon Dioxide with a Borane
Abstract
Nickel hydride with a diphosphinite-based ligand catalyzes the highly efficient reduction of CO(2) with catecholborane, and the hydrolysis of the resulting methoxyboryl species produces CH(3)OH in good yield. The mechanism involves a nickel formate, formaldehyde, and a nickel methoxide as different reduced stages for CO(2). The reaction may also be catalyzed by an air-stable nickel formate.
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Citations
Cites
Darensbourg, D. J. (2007) · Chemical Reviews · doi:10.1021/cr068363q · Cited by 1,593
Cited by
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Goeppert, A., Czaun, M., Jones, J.-P., Surya Prakash, G. K., & Olah, G. A. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00122b · Cited by 1,528
Klankermayer, J., Wesselbaum, S., Beydoun, K., & Leitner, W. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201507458 · Cited by 856
Sustainable conversion of carbon dioxide: the advent of organocatalysis
Fiorani, G., Guo, W., & Kleij, A. W. (2015) · Green Chemistry · doi:10.1039/c4gc01959h · Cited by 658
Tlili, A., Blondiaux, E., Frogneux, X., & Cantat, T. (2015) · Green Chemistry · doi:10.1039/c4gc01614a · Cited by 403
New Strategies for the Preparation of Sinter‐Resistant Metal‐Nanoparticle‐Based Catalysts
Wang, L., Wang, L., Meng, X., & Xiao, F. (2019) · Advanced Materials · doi:10.1002/adma.201901905 · Cited by 384
Metadata
- Authors
- Chakraborty, S., Zhang, J., Krause, J. A., & Guan, H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-06-14
- Volume
- 132
- Issue
- 26
- Pages
- 8872-8873
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2089307567
- Cited by
- 432
- References
- 1
- FWCI
- 15.49
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
