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Multistimuli Two-Color Luminescence Switching via Different Slip-Stacking of Highly Fluorescent Molecular Sheets
Abstract
Color tuning and switching of the solid-state luminescence of organic materials are attractive subjects for both the fundamental research and practical applications such as optical recording. We report herein cyanostilbene-based highly luminescent molecular sheets which exhibit two-color fluorescence switching in response to pressure, temperature, and solvent vapor. The origin for the multistimuli luminescence switching is the two-directional shear-sliding capability of molecular sheets, which are formed via intermolecular multiple C-H···N and C-H···O hydrogen bonds. The resulting two distinctive crystal phases are promoted by different modes of local dipole coupling, which cause a substantial alternation of π-π overlap. These changes can be directly correlated with the subsequent intermolecular excitonic and excimeric coupling in both phases, as demonstrated by an in-depth theory-assisted spectroscopic and structural study. Finally, we have prepared a first device demonstrator for rewritable fluorescent optical recording media which showed multistimuli luminescence tuning with fast response. Our multistimuli responsive system is unique in terms of the slip-stacking of molecular sheets and thus provides a novel concept of rewritable fluorescent optical recording media.
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Metadata
- Authors
- Yoon, S.-J., Chung, J. W., Gierschner, J., Kim, K. S., Choi, M.-G., Kim, D., & Park, S. Y.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-09-14
- Volume
- 132
- Issue
- 39
- Pages
- 13675-13683
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2050206869
- Cited by
- 950
- References
- 1
- FWCI
- 25.02
- Type
- journal article
- Language
- en
- Open access
- closed
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