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Tunable Photocatalytic Selectivity of Hollow TiO2 Microspheres Composed of Anatase Polyhedra with Exposed {001} Facets
Abstract
A fluoride mediated self-transformation method is proposed for the synthesis of hollow TiO(2) microspheres (HTS) composed of anatase polyhedra with exposed ca. 20% {001} facets. Importantly, HTS exhibit tunable photocatalytic selectivity in decomposing azo dyes in water. The fluorinated HTS show preferential decomposition of methyl orange (MO) in comparison to methylene blue (MB). In contrast, the surface-modified HTS by either NaOH washing or calcinations at 600 degrees C favor decomposition of MB over MO. The surface chemistry and the surface structure at the atomic level are key factors in tuning the adsorption selectivity and, consequently, photocatalytic selectivity of HTS toward azo dyes.
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Cites
Electrochemical Photolysis of Water at a Semiconductor Electrode
FUJISHIMA, A., & HONDA, K. (1972) · Nature · doi:10.1038/238037a0 · Cited by 34,169
Environmental applications of semiconductor photocatalysis
Hoffmann, M. R., Martin, S. T., Choi, W., & Bahnemann, D. W. (1995) · Chemical Reviews · doi:10.1021/cr00033a004 · Cited by 18,495
Cited by
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Nakata, K., & Fujishima, A. (2012) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2012.06.001 · Cited by 3,651
Graphene-based semiconductor photocatalysts
Xiang, Q., Yu, J., & Jaroniec, M. (2012) · Chem. Soc. Rev. · doi:10.1039/c1cs15172j · Cited by 2,730
Self-citationXiang, Q., Yu, J., & Jaroniec, M. (2012) · Journal of the American Chemical Society · doi:10.1021/ja302846n · Cited by 2,360
Self-citationAjmal, A., Majeed, I., Malik, R. N., Idriss, H., & Nadeem, M. A. (2014) · RSC Adv. · doi:10.1039/c4ra06658h · Cited by 1,485
Facet Effect of Single-Crystalline Ag3PO4 Sub-microcrystals on Photocatalytic Properties
Bi, Y., Ouyang, S., Umezawa, N., Cao, J., & Ye, J. (2011) · Journal of the American Chemical Society · doi:10.1021/ja2002132 · Cited by 1,316
Metadata
- Authors
- Liu, S., Yu, J., & Jaroniec, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-08-05
- Volume
- 132
- Issue
- 34
- Pages
- 11914-11916
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1972186003
- Cited by
- 1,011
- References
- 2
- FWCI
- 51.15
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, S., Yu, J., & Jaroniec, M. (2010). Tunable Photocatalytic Selectivity of Hollow TiO2 Microspheres Composed of Anatase Polyhedra with Exposed {001} Facets. Journal of the American Chemical Society. https://doi.org/10.1021/ja105283s
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