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Enhanced Electrochemical Lithium Storage by Graphene Nanoribbons
Abstract
Herein, we report the electrochemical Li intake capacity of carbonaceous one-dimensional graphene nanoribbons (GNRs) obtained by unzipping pristine multiwalled carbon nanotubes (MWCNTs). We have found that nanotubes with diameters of approximately 50 nm present a smaller reversible capacity than conventional mesocarbon microbead (MCMB) powder. Reduced GNRs improve the capacity only marginally over the MCMB reference but present a lower Coulombic efficiency as well as a higher capacity loss per cycle. Oxidized GNRs (ox-GNRs) outperform all of the other materials studied here in terms of energy density. They present a first charge capacity of approximately 1400 mA h g(-1) with a low Coulombic efficiency for the first cycle (approximately 53%). The reversible capacity of ox-GNRs is in the range of 800 mA h g(-1), with a capacity loss per cycle of approximately 3% for early cycles and a decreasing loss rate for subsequent cycles.
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Metadata
- Authors
- Bhardwaj, T., Antic, A., Pavan, B., Barone, V., & Fahlman, B. D.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-08-23
- Volume
- 132
- Issue
- 36
- Pages
- 12556-12558
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2064753851
- Cited by
- 273
- References
- 25
- FWCI
- 20.18
- Type
- journal article
- Language
- en
- Open access
- closed
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