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Synergistic Catalysis of Au@Ag Core−Shell Nanoparticles Stabilized on Metal−Organic Framework
Abstract
For the first time, this work presents Au@Ag core-shell nanoparticles (NPs) immobilized on a metal-organic framework (MOF) by a sequential deposition-reduction method. The small-size Au@Ag NPs reveal the restriction effects of the pore/surface structure in the MOF. The modulation of the Au/Ag ratio can tune the composition and a reversed Au/Ag deposition sequence changes the structure of Au-Ag NPs, while a posttreatment process transforms the core-shell NPs to a AuAg alloy. Catalytic studies show a strong bimetallic synergistic effect of core-shell structured Au@Ag NPs, which have much higher catalytic activities than alloy and monometallic NPs.
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Cites
Nanoalloys: From Theory to Applications of Alloy Clusters and Nanoparticles
Ferrando, R., Jellinek, J., & Johnston, R. L. (2008) · Chemical Reviews · doi:10.1021/cr040090g · Cited by 3,690
Horike, S., Shimomura, S., & Kitagawa, S. (2009) · Nature Chemistry · doi:10.1038/nchem.444 · Cited by 2,486
Cited by
Metal–organic frameworks as platforms for clean energy
Li, S.-L., & Xu, Q. (2013) · Energy & Environmental Science · doi:10.1039/c3ee40507a · Cited by 970
State of the art in gold nanoparticle synthesis
Zhao, P., Li, N., & Astruc, D. (2013) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2012.09.002 · Cited by 964
Zhan, W.-W., Kuang, Q., Zhou, J.-Z., Kong, X.-J., Xie, Z.-X., & Zheng, L.-S. (2013) · Journal of the American Chemical Society · doi:10.1021/ja311085e · Cited by 803
Synthesis and catalytic properties of bimetallic nanomaterials with various architectures
Liu, X., Wang, D., & Li, Y. (2012) · Nano Today · doi:10.1016/j.nantod.2012.08.003 · Cited by 538
Tailored crystalline microporous materials by post-synthesis modification
Valtchev, V., Majano, G., Mintova, S., & Pérez-Ramírez, J. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35196j · Cited by 478
Metadata
- Authors
- Jiang, H.-L., Akita, T., Ishida, T., Haruta, M., & Xu, Q.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-01-07
- Volume
- 133
- Issue
- 5
- Pages
- 1304-1306
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2314213609
- Cited by
- 931
- References
- 2
- FWCI
- 45.91
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jiang, H.-L., Akita, T., Ishida, T., Haruta, M., & Xu, Q. (2011). Synergistic Catalysis of Au@Ag Core−Shell Nanoparticles Stabilized on Metal−Organic Framework. Journal of the American Chemical Society. https://doi.org/10.1021/ja1099006
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
