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Synergistic Catalysis of Au@Ag Core−Shell Nanoparticles Stabilized on Metal−Organic Framework
Abstract
For the first time, this work presents Au@Ag core-shell nanoparticles (NPs) immobilized on a metal-organic framework (MOF) by a sequential deposition-reduction method. The small-size Au@Ag NPs reveal the restriction effects of the pore/surface structure in the MOF. The modulation of the Au/Ag ratio can tune the composition and a reversed Au/Ag deposition sequence changes the structure of Au-Ag NPs, while a posttreatment process transforms the core-shell NPs to a AuAg alloy. Catalytic studies show a strong bimetallic synergistic effect of core-shell structured Au@Ag NPs, which have much higher catalytic activities than alloy and monometallic NPs.
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Metadata
- Authors
- Jiang, H.-L., Akita, T., Ishida, T., Haruta, M., & Xu, Q.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-01-07
- Volume
- 133
- Issue
- 5
- Pages
- 1304-1306
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2314213609
- Cited by
- 931
- References
- 44
- FWCI
- 45.91
- Type
- journal article
- Language
- en
- Open access
- closed
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