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Hierarchical Helical Assembly of Conjugated Poly(3-hexylthiophene)-block-poly(3-triethylene glycol thiophene) Diblock Copolymers
Abstract
We report on the solution-state assembly of all-conjugated polythiophene diblock copolymers containing nonpolar (hexyl) and polar (triethylene glycol) side chains. The polar substituents provide a large contrast in solubility, enabling formation of stably suspended crystalline fibrils even under very poor solvent conditions for the poly(3-hexylthiophene) block. For appropriate block ratios, complexation of the triethylene glycol side chains with added potassium ions drives the formation of helical nanowires that further bundle into superhelical structures.
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Citations
Cited by
Yashima, E., Ousaka, N., Taura, D., Shimomura, K., Ikai, T., & Maeda, K. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00354 · Cited by 2,004
Tritschler, U., Pearce, S., Gwyther, J., Whittell, G. R., & Manners, I. (2017) · Macromolecules · doi:10.1021/acs.macromol.6b02767 · Cited by 375
Gilroy, J. B., Rupar, P. A., Whittell, G. R., Chabanne, L., Terrill, N. J., Winnik, M. A., Manners, I., & Richardson, R. M. (2011) · Journal of the American Chemical Society · doi:10.1021/ja207417z · Cited by 97
Metadata
- Authors
- Lee, E., Hammer, B., Kim, J.-K., Page, Z., Emrick, T., & Hayward, R. C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-06-16
- Volume
- 133
- Issue
- 27
- Pages
- 10390-10393
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2060022677
- Cited by
- 227
- References
- 0
- FWCI
- 12.39
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Hierarchical Helical Assembly of Conjugated Poly(3-hexylthiophene)-block-poly(3-triethylene glycol thiophene) Diblock Copolymers. https://app.cochat.ai/papers/10.1021/ja2038547
- The paper
- Lee, E., Hammer, B., Kim, J.-K., Page, Z., Emrick, T., & Hayward, R. C. (2011). Hierarchical Helical Assembly of Conjugated Poly(3-hexylthiophene)-block-poly(3-triethylene glycol thiophene) Diblock Copolymers. Journal of the American Chemical Society. https://doi.org/10.1021/ja2038547
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
