The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Capture of Volatile Iodine, a Gaseous Fission Product, by Zeolitic Imidazolate Framework-8
Abstract
Here we present detailed structural evidence of captured molecular iodine (I(2)), a volatile gaseous fission product, within the metal-organic framework ZIF-8 [zeolitic imidazolate framework-8 or Zn(2-methylimidazolate)(2)]. There is worldwide interest in the effective capture and storage of radioiodine, as it is both produced from nuclear fuel reprocessing and also commonly released in nuclear reactor accidents. Insights from multiple complementary experimental and computational probes were combined to locate I(2) molecules crystallographically inside the sodalite cages of ZIF-8 and to understand the capture of I(2) via bonding with the framework. These structural tools included high-resolution synchrotron powder X-ray diffraction, pair distribution function analysis, and molecular modeling simulations. Additional tests indicated that extruded ZIF-8 pellets perform on par with ZIF-8 powder and are industrially suitable for I(2) capture.
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Cites
Fast Parallel Algorithms for Short-Range Molecular Dynamics
Plimpton, S. (1995) · Journal of Computational Physics · doi:10.1006/jcph.1995.1039 · Cited by 44,721
Cited by
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Synthesis of novel nanomaterials and their application in efficient removal of radionuclides
Wang, X., Chen, L., Wang, L., Fan, Q., Pan, D., Li, J., Chi, F., Xie, Y., Yu, S., Xiao, C., et al. (2019) · Science China Chemistry · doi:10.1007/s11426-019-9492-4 · Cited by 365
Competitive I2 Sorption by Cu-BTC from Humid Gas Streams
Sava, D. F., Chapman, K. W., Rodriguez, M. A., Greathouse, J. A., Crozier, P. S., Zhao, H., Chupas, P. J., & Nenoff, T. M. (2013) · Chemistry of Materials · doi:10.1021/cm401762g · Cited by 363
Self-citationSubrahmanyam, K. S., Malliakas, C. D., Sarma, D., Armatas, G. S., Wu, J., & Kanatzidis, M. G. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b09110 · Cited by 193
Ionic liquids and deep eutectic solvents in wastewater treatment: recent endeavours
Sarkar, A., & Pandey, S. (2024) · International Journal of Environmental Science and Technology · doi:10.1007/s13762-023-04865-1 · Cited by 14
Metadata
- Authors
- Sava, D. F., Rodriguez, M. A., Chapman, K. W., Chupas, P. J., Greathouse, J. A., Crozier, P. S., & Nenoff, T. M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-07-26
- Volume
- 133
- Issue
- 32
- Pages
- 12398-12401
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2064076126
- Cited by
- 725
- References
- 1
- FWCI
- 16.20
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sava, D. F., Rodriguez, M. A., Chapman, K. W., Chupas, P. J., Greathouse, J. A., Crozier, P. S., & Nenoff, T. M. (2011). Capture of Volatile Iodine, a Gaseous Fission Product, by Zeolitic Imidazolate Framework-8. Journal of the American Chemical Society. https://doi.org/10.1021/ja204757x
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