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Microporous Polycarbazole with High Specific Surface Area for Gas Storage and Separation
Abstract
Microporous polycarbazole via straightforward carbazole-based oxidative coupling polymerization is reported. The synthesis route exhibits cost-effective advantages, which are essential for scale-up preparation. The Brunauer-Emmett-Teller specific surface area for obtained polymer is up to 2220 m(2) g(-1). Gas (H(2) and CO(2)) adsorption isotherms show that its hydrogen storage can reach to 2.80 wt % (1.0 bar and 77 K) and the uptake capacity for carbon dioxide is up to 21.2 wt % (1.0 bar and 273 K), which show a promising potential for clean energy application and environmental field. Furthermore, the high selectivity toward CO(2) over N(2) and CH(4) makes the obtained polymer possess potential application in gas separation.
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Sing, K. S. W. (1985) · Pure and Applied Chemistry · doi:10.1351/pac198557040603 · Cited by 24,485
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Metadata
- Authors
- Chen, Q., Luo, M., Hammershøj, P., Zhou, D., Han, Y., Laursen, B. W., Yan, C.-G., & Han, B.-H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-03-30
- Volume
- 134
- Issue
- 14
- Pages
- 6084-6087
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2001044107
- Cited by
- 704
- References
- 1
- FWCI
- 28.09
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, Q., Luo, M., Hammershøj, P., Zhou, D., Han, Y., Laursen, B. W., Yan, C.-G., & Han, B.-H. (2012). Microporous Polycarbazole with High Specific Surface Area for Gas Storage and Separation. Journal of the American Chemical Society. https://doi.org/10.1021/ja300438w
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