The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Li–O2 Battery with a Dimethylformamide Electrolyte
Abstract
Stability of the electrolyte toward reduced oxygen species generated at the cathode is a crucial challenge for the rechargeable nonaqueous Li-O(2) battery. Here, we investigate dimethylformamide as the basis of an electrolyte. Although reactions at the O(2) cathode on the first discharge-charge cycle are dominated by reversible Li(2)O(2) formation/decomposition, there is also electrolyte decomposition, which increases on cycling. The products of decomposition at the cathode on discharge are Li(2)O(2), Li(2)CO(3), HCO(2)Li, CH(3)CO(2)Li, NO, H(2)O, and CO(2). Li(2)CO(3) accumulates in the electrode with cycling. The stability of dimethylformamide toward reduced oxygen species is insufficient for its use in the rechargeable nonaqueous Li-O(2) battery.
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Citations
Cites
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Self-citation
Cited by
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Smaller Sulfur Molecules Promise Better Lithium–Sulfur Batteries
Xin, S., Gu, L., Zhao, N.-H., Yin, Y.-X., Zhou, L.-J., Guo, Y.-G., & Wan, L.-J. (2012) · Journal of the American Chemical Society · doi:10.1021/ja308170k · Cited by 1,644
From lithium to sodium: Cell chemistry of room temperature sodium–air and sodium–sulfur batteries
Adelhelm, P., Hartmann, P., Bender, C. L., Busche, M., Eufinger, C., & Janek, J. (2015) · Beilstein Journal of Nanotechnology · doi:10.3762/bjnano.6.105 · Cited by 478
Flammability of Li-Ion Battery Electrolytes: Flash Point and Self-Extinguishing Time Measurements
Hess, S., Wohlfahrt-Mehrens, M., & Wachtler, M. (2015) · Journal of The Electrochemical Society · doi:10.1149/2.0121502jes · Cited by 451
Critical Challenges in Rechargeable Aprotic Li–O2 Batteries
Feng, N., He, P., & Zhou, H. (2016) · Advanced Energy Materials · doi:10.1002/aenm.201502303 · Cited by 423
Metadata
- Authors
- Chen, Y., Freunberger, S. A., Peng, Z., Bardé, F., & Bruce, P. G.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-05-01
- Volume
- 134
- Issue
- 18
- Pages
- 7952-7957
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2313247439
- Cited by
- 387
- References
- 1
- FWCI
- 29.71
- Type
- journal article
- Language
- en
- Open access
- closed
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