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How Water Fosters a Remarkable 5-Fold Increase in Low-Pressure CO2 Uptake within Mesoporous MIL-100(Fe)
Abstract
The uptake and adsorption enthalpy of carbon dioxide at 0.2 bar have been studied in three different topical porous MOF samples, HKUST-1, UiO-66(Zr), and MIL-100(Fe), after having been pre-equilibrated under different relative humidities (3, 10, 20, 40%) of water vapor. If in the case of microporous UiO-66, CO(2) uptake remained similar whatever the relative humidity, and correlations were difficult for microporous HKUST-1 due to its relative instability toward water vapor. In the case of MIL-100(Fe), a remarkable 5-fold increase in CO(2) uptake was observed with increasing RH, up to 105 mg g(-1) CO(2) at 40% RH, in parallel with a large decrease in enthalpy measured. Cycling measurements show slight differences for the initial three cycles and complete reversibility with further cycles. These results suggest an enhanced solubility of CO(2) in the water-filled mesopores of MIL-100(Fe).
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Hansen, J., Ruedy, R., Sato, M., & Lo, K. (2010) · Reviews of Geophysics · doi:10.1029/2010rg000345 · Cited by 3,081
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Burtch, N. C., Jasuja, H., & Walton, K. S. (2014) · Chemical Reviews · doi:10.1021/cr5002589 · Cited by 2,730
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Canivet, J., Fateeva, A., Guo, Y., Coasne, B., & Farrusseng, D. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00078a · Cited by 1,444
CO2 Capture and Separations Using MOFs: Computational and Experimental Studies
Yu, J., Xie, L.-H., Li, J.-R., Ma, Y., Seminario, J. M., & Balbuena, P. B. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00626 · Cited by 1,047
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Kalmutzki, M. J., Diercks, C. S., & Yaghi, O. M. (2018) · Advanced Materials · doi:10.1002/adma.201704304 · Cited by 772
Understanding the Effect of Water on CO2 Adsorption
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Metadata
- Authors
- Soubeyrand-Lenoir, E., Vagner, C., Yoon, J. W., Bazin, P., Ragon, F., Hwang, Y. K., Serre, C., Chang, J.-S., & Llewellyn, P. L.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-06-11
- Volume
- 134
- Issue
- 24
- Pages
- 10174-10181
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2323873465
- Cited by
- 234
- References
- 1
- FWCI
- 10.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Soubeyrand-Lenoir, E., Vagner, C., Yoon, J. W., Bazin, P., Ragon, F., Hwang, Y. K., Serre, C., Chang, J.-S., & Llewellyn, P. L. (2012). How Water Fosters a Remarkable 5-Fold Increase in Low-Pressure CO2 Uptake within Mesoporous MIL-100(Fe). Journal of the American Chemical Society. https://doi.org/10.1021/ja302787x
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