The DOI matches its Crossref record; 31 of the 31 references it cites were found in a registry or an index.
Toward an Ideal Polymer Binder Design for High-Capacity Battery Anodes
Open accessAbstract
The dilemma of employing high-capacity battery materials and maintaining the electronic and mechanical integrity of electrodes demands novel designs of binder systems. Here, we developed a binder polymer with multifunctionality to maintain high electronic conductivity, mechanical adhesion, ductility, and electrolyte uptake. These critical properties are achieved by designing polymers with proper functional groups. Through synthesis, spectroscopy, and simulation, electronic conductivity is optimized by tailoring the key electronic state, which is not disturbed by further modifications of side chains. This fundamental allows separated optimization of the mechanical and swelling properties without detrimental effect on electronic property. Remaining electronically conductive, the enhanced polarity of the polymer greatly improves the adhesion, ductility, and more importantly, the electrolyte uptake to the levels of those available only in nonconductive binders before. We also demonstrate directly the performance of the developed conductive binder by achieving full-capacity cycling of silicon particles without using any conductive additive.
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Cites
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Self-citationNanocomposite polymer electrolytes for lithium batteries
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Cited by
Silicon‐Based Anodes for Lithium‐Ion Batteries: From Fundamentals to Practical Applications
Feng, K., Li, M., Liu, W., Kashkooli, A. G., Xiao, X., Cai, M., & Chen, Z. (2018) · Small · doi:10.1002/smll.201702737 · Cited by 1,042
Self-citationChen, H., Ling, M., Hencz, L., Ling, H. Y., Li, G., Lin, Z., Liu, G., & Zhang, S. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00241 · Cited by 958
Self-citationNanostructured conductive polymers for advanced energy storage
Shi, Y., Peng, L., Ding, Y., Zhao, Y., & Yu, G. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00362h · Cited by 932
Designing polymers for advanced battery chemistries
Lopez, J., Mackanic, D. G., Cui, Y., & Bao, Z. (2019) · Nature Reviews Materials · doi:10.1038/s41578-019-0103-6 · Cited by 894
The emerging era of supramolecular polymeric binders in silicon anodes
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Metadata
- Authors
- Wu, M., Xiao, X., Vukmirovic, N., Xun, S., Das, P. K., Song, X., Olalde-Velasco, P., Wang, D., Weber, A. Z., Wang, L.-W., Battaglia, V. S., Yang, W., & Liu, G.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-07-31
- Volume
- 135
- Issue
- 32
- Pages
- 12048-12056
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2170943742
- Cited by
- 398
- References
- 31
- FWCI
- 17.37
- Type
- journal article
- Language
- en
- Open access
- green
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- Wu, M., Xiao, X., Vukmirovic, N., Xun, S., Das, P. K., Song, X., Olalde-Velasco, P., Wang, D., Weber, A. Z., Wang, L.-W., Battaglia, V. S., Yang, W., & Liu, G. (2013). Toward an Ideal Polymer Binder Design for High-Capacity Battery Anodes. Journal of the American Chemical Society. https://doi.org/10.1021/ja4054465
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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