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Programmed Pore Architectures in Modular Quaternary Metal–Organic Frameworks
Abstract
To generate metal-organic frameworks (MOFs) that are complex and modular yet well ordered, we present a strategy employing a family of three topologically distinct linkers that codes for the assembly of a highly porous quaternary MOF. By introducing substituted analogues of the ligands, a set of eight isoreticular frameworks is delivered, with the MOF structure systematically varied while the topology is maintained. To combat randomness and disorder, the substitution patterns of the ligands are designed to be compatible with their crystallographic site symmetries. MOFs produced in this way feature "programmed pores"--multiple functional groups compartmentalized in a predetermined array within a periodic lattice--and are capable of complex functional behavior. In these examples unconventional CO2 sorption trends, including capacity enhancements close to 100%, emerge from synergistic effects. Future PP-MOFs may be capable of enzyme-like heterogeneous catalysis and ultraselective adsorption.
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Cites
Large-scale screening of hypothetical metal–organic frameworks
Wilmer, C. E., Leaf, M., Lee, C. Y., Farha, O. K., Hauser, B. G., Hupp, J. T., & Snurr, R. Q. (2012) · Nature Chemistry · doi:10.1038/nchem.1192 · Cited by 1,439
Cited by
From fundamentals to applications: a toolbox for robust and multifunctional MOF materials
Kirchon, A., Feng, L., Drake, H. F., Joseph, E. A., & Zhou, H.-C. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00688a · Cited by 1,448
“Heterogeneity within Order” in Metal–Organic Frameworks
Furukawa, H., Müller, U., & Yaghi, O. M. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201410252 · Cited by 549
A reticular chemistry guide for the design of periodic solids
Jiang, H., Alezi, D., & Eddaoudi, M. (2021) · Nature Reviews Materials · doi:10.1038/s41578-021-00287-y · Cited by 432
Li, B., Leng, K., Zhang, Y., Dynes, J. J., Wang, J., Hu, Y., Ma, D., Shi, Z., Zhu, L., Zhang, D., et al. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b01352 · Cited by 264
Metadata
- Authors
- Liu, L., Konstas, K., Hill, M. R., & Telfer, S. G.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-11-13
- Volume
- 135
- Issue
- 47
- Pages
- 17731-17734
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2312965003
- Cited by
- 195
- References
- 1
- FWCI
- 8.64
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, L., Konstas, K., Hill, M. R., & Telfer, S. G. (2013). Programmed Pore Architectures in Modular Quaternary Metal–Organic Frameworks. Journal of the American Chemical Society. https://doi.org/10.1021/ja4100244
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
