The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Visible Light-Driven Pure Water Splitting by a Nature-Inspired Organic Semiconductor-Based System
Open accessAbstract
For the first time, it is demonstrated that the robust organic semiconductor g-C3N4 can be integrated into a nature-inspired water splitting system, analogous to PSII and PSI in natural photosynthesis. Two parallel systems have been developed for overall water splitting under visible light involving graphitic carbon nitride with two different metal oxides, BiVO4 and WO3. Consequently, both hydrogen and oxygen can be evolved in an ideal ratio of 2:1, and evolution rates in both systems have been found to be dependent on pH, redox mediator concentration, and mass ratio between the two photocatalysts, leading to a stable and reproducible H2 and O2 evolution rate at 36 and 18 μmol h(-1) g(-1) from water over 14 h. Our findings demonstrate g-C3N4 can serve as a multifunctional robust photocatalyst, which could also be used in other systems such as PEC cells or coupled solar cell systems.
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Cites
Electrochemical Photolysis of Water at a Semiconductor Electrode
FUJISHIMA, A., & HONDA, K. (1972) · Nature · doi:10.1038/238037a0 · Cited by 34,169
Nanostructured Tungsten Oxide – Properties, Synthesis, and Applications
Zheng, H., Ou, J. Z., Strano, M. S., Kaner, R. B., Mitchell, A., & Kalantar‐zadeh, K. (2011) · Advanced Functional Materials · doi:10.1002/adfm.201002477 · Cited by 1,479
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Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Conquering the Hypoxia Limitation for Photodynamic Therapy
Wan, Y., Fu, L., Li, C., Lin, J., & Huang, P. (2021) · Advanced Materials · doi:10.1002/adma.202103978 · Cited by 705
Z‐Scheme Photocatalytic Systems for Solar Water Splitting
Ng, B., Putri, L. K., Kong, X. Y., Teh, Y. W., Pasbakhsh, P., & Chai, S. (2020) · Advanced Science · doi:10.1002/advs.201903171 · Cited by 533
Phototherapy in cancer treatment: strategies and challenges
Cai, Y., Chai, T., Nguyen, W., Liu, J., Xiao, E., Ran, X., Ran, Y., Du, D., Chen, W., & Chen, X. (2025) · Signal Transduction and Targeted Therapy · doi:10.1038/s41392-025-02140-y · Cited by 453
Metadata
- Authors
- Martin, D. J., Reardon, P. J. T., Moniz, S. J. A., & Tang, J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-08-26
- Volume
- 136
- Issue
- 36
- Pages
- 12568-12571
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1974659797
- Cited by
- 556
- References
- 2
- FWCI
- 16.92
- Type
- journal article
- Language
- en
- Open access
- hybrid
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