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In Situ Synthesis of MOF Membranes on ZnAl-CO3 LDH Buffer Layer-Modified Substrates
Abstract
We develop here a urea hydrolysis method to in situ prepare asymmetric ZnAl-CO3 layered double hydroxide (LDH) buffer layers with various stable equilibrium morphology on porous Al2O3 substrates. In particular it is found that well-intergrown ZIF-8 membranes can be directly synthesized on the ZnAl-CO3 LDH buffer layer-modified substrates, owing to the specific metal-imidazole interaction between ZnAl-CO3 LDHs and ZIF-8. Other Zn-based MOF membranes, like ZIF-7 and ZIF-90, can also be synthesized with this method. Our finding demonstrates that LDH buffer layer represents a new concept for substrate modification.
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Citations
Cited by
Dai, H., Yuan, X., Jiang, L., Wang, H., Zhang, J., Zhang, J., & Xiong, T. (2021) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2021.213985 · Cited by 503
Li, Z., Shao, M., Zhou, L., Zhang, R., Zhang, C., Wei, M., Evans, D. G., & Duan, X. (2016) · Advanced Materials · doi:10.1002/adma.201505086 · Cited by 498
Microporous framework membranes for precise molecule/ion separations
Dou, H., Xu, M., Wang, B., Zhang, Z., Wen, G., Zheng, Y., Luo, D., Zhao, L., Yu, A., Zhang, L., et al. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00552e · Cited by 371
Ultrathin metal–organic framework membrane production by gel–vapour deposition
Li, W., Su, P., Li, Z., Xu, Z., Wang, F., Ou, H., Zhang, J., Zhang, G., & Zeng, E. (2017) · Nature Communications · doi:10.1038/s41467-017-00544-1 · Cited by 353
Ceramic-based membranes for water and wastewater treatment
He, Z., Lyu, Z., Gu, Q., Zhang, L., & Wang, J. (2019) · Colloids and Surfaces A: Physicochemical and Engineering Aspects · doi:10.1016/j.colsurfa.2019.05.074 · Cited by 323
Metadata
- Authors
- Liu, Y., Wang, N., Pan, J. H., Steinbach, F., & Caro, J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-10-03
- Volume
- 136
- Issue
- 41
- Pages
- 14353-14356
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2327679667
- Cited by
- 225
- References
- 0
- FWCI
- 5.64
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, Y., Wang, N., Pan, J. H., Steinbach, F., & Caro, J. (2014). In Situ Synthesis of MOF Membranes on ZnAl-CO3 LDH Buffer Layer-Modified Substrates. Journal of the American Chemical Society. https://doi.org/10.1021/ja507408s
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