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Quest for Anionic MOF Membranes: Continuous sod-ZMOF Membrane with CO2 Adsorption-Driven Selectivity
Abstract
We report the fabrication of the first continuous zeolite-like metal-organic framework (ZMOF) thin-film membrane. A pure phase sod-ZMOF, sodalite topology, membrane was grown and supported on a porous alumina substrate using a solvothermal crystallization method. The absence of pinhole defects in the film was confirmed and supported by the occurrence of quantifiable time-lags, for all studied gases, during constant volume/variable pressure permeation tests. For both pure and mixed gas feeds, the sod-ZMOF-1 membrane exhibits favorable permeation selectivity toward carbon dioxide over relevant industrial gases such as H2, N2, and CH4, and it is mainly governed by favorable CO2 adsorption.
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Cited by
The chemistry of metal–organic frameworks for CO2 capture, regeneration and conversion
Trickett, C. A., Helal, A., Al-Maythalony, B. A., Yamani, Z. H., Cordova, K. E., & Yaghi, O. M. (2017) · Nature Reviews Materials · doi:10.1038/natrevmats.2017.45 · Cited by 1,524
Self-citationCO2 Capture and Separations Using MOFs: Computational and Experimental Studies
Yu, J., Xie, L.-H., Li, J.-R., Ma, Y., Seminario, J. M., & Balbuena, P. B. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00626 · Cited by 1,047
Porous metal-organic frameworks for gas storage and separation: Status and challenges
Li, H., Li, L., Lin, R.-B., Zhou, W., Zhang, Z., Xiang, S., & Chen, B. (2019) · EnergyChem · doi:10.1016/j.enchem.2019.100006 · Cited by 891
Liu, X., Demir, N. K., Wu, Z., & Li, K. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b02276 · Cited by 802
Liu, J., & Wöll, C. (2017) · Chemical Society Reviews · doi:10.1039/c7cs00315c · Cited by 698
Metadata
- Authors
- Al-Maythalony, B. A., Shekhah, O., Swaidan, R., Belmabkhout, Y., Pinnau, I., & Eddaoudi, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-01-28
- Volume
- 137
- Issue
- 5
- Pages
- 1754-1757
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2313052804
- Cited by
- 160
- References
- 0
- FWCI
- 22.88
- Type
- journal article
- Language
- en
- Open access
- closed
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- Al-Maythalony, B. A., Shekhah, O., Swaidan, R., Belmabkhout, Y., Pinnau, I., & Eddaoudi, M. (2015). Quest for Anionic MOF Membranes: Continuous sod-ZMOF Membrane with CO2 Adsorption-Driven Selectivity. Journal of the American Chemical Society. https://doi.org/10.1021/ja511495j
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