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Graphdiyne Oxides as Excellent Substrate for Electroless Deposition of Pd Clusters with High Catalytic Activity
Abstract
Graphdiyne (GDY), a novel kind of two-dimensional carbon allotrope consisting of sp- and sp(2)-hybridized carbon atoms, is found to be able to serve as the reducing agent and stabilizer for electroless deposition of highly dispersed Pd nanoparticles owing to its low reduction potential and highly conjugated electronic structure. Furthermore, we observe that graphdiyne oxide (GDYO), the oxidation form of GDY, can be used as an even excellent substrate for electroless deposition of ultrafine Pd clusters to form Pd/GDYO nanocomposite that exhibits a high catalytic performance toward the reduction of 4-nitrophenol. The high catalytic performance is considered to benefit from the rational design and electroless deposition of active metal catalysts with GDYO as the support.
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Cited by
Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution
Xue, Y., Huang, B., Yi, Y., Guo, Y., Zuo, Z., Li, Y., Jia, Z., Liu, H., & Li, Y. (2018) · Nature Communications · doi:10.1038/s41467-018-03896-4 · Cited by 1,011
Self-citationHighly Efficient and Selective Generation of Ammonia and Hydrogen on a Graphdiyne-Based Catalyst
Hui, L., Xue, Y., Yu, H., Liu, Y., Fang, Y., Xing, C., Huang, B., & Li, Y. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b03004 · Cited by 587
Self-citationSynthesis and Properties of 2D Carbon—Graphdiyne
Jia, Z., Li, Y., Zuo, Z., Liu, H., Huang, C., & Li, Y. (2017) · Accounts of Chemical Research · doi:10.1021/acs.accounts.7b00205 · Cited by 565
Self-citation2D graphdiyne: An emerging carbon material
Fang, Y., Liu, Y., Qi, L., Xue, Y., & Li, Y. (2022) · Chemical Society Reviews · doi:10.1039/d1cs00592h · Cited by 520
Self-citationRobust Superhydrophobic Foam: A Graphdiyne‐Based Hierarchical Architecture for Oil/Water Separation
Gao, X., Zhou, J., Du, R., Xie, Z., Deng, S., Liu, R., Liu, Z., & Zhang, J. (2016) · Advanced Materials · doi:10.1002/adma.201504407 · Cited by 513
Metadata
- Authors
- Qi, H., Yu, P., Wang, Y., Han, G., Liu, H., Yi, Y., Li, Y., & Mao, L.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-04-15
- Volume
- 137
- Issue
- 16
- Pages
- 5260-5263
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2317113583
- Cited by
- 393
- References
- 0
- FWCI
- 17.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Qi, H., Yu, P., Wang, Y., Han, G., Liu, H., Yi, Y., Li, Y., & Mao, L. (2015). Graphdiyne Oxides as Excellent Substrate for Electroless Deposition of Pd Clusters with High Catalytic Activity. Journal of the American Chemical Society. https://doi.org/10.1021/ja5131337
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