The DOI matches its Crossref record; 46 of the 46 references it cites were found in a registry or an index.
Highly Efficient and Selective Generation of Ammonia and Hydrogen on a Graphdiyne-Based Catalyst
Abstract
The emergence of zerovalent atom catalysts has been highly attractive for catalytic science. For many years, scientists have explored the stability of zerovalent atom catalysts and demonstrated their unique properties. Here, we describe an atom catalyst (AC) with atomically dispersed zerovalent molybdenum atoms on graphdiyne (Mo 0 /GDY) with a high mass content of Mo atoms (up to 7.5 wt %) that was synthesized via a facile and scalable process. The catalyst shows both excellent selectivity and activity in the electrochemical reduction of nitrogen and in the hydrogen evolution reaction in aqueous solutions at room temperature and pressure. It is noted that this catalyst is the first bifunctional AC for highly efficient and selective ammonia and hydrogen generation. The catalytic process of our catalyst is well understood, the structure is defined, and the performance is excellent, providing a solid foundation for the generation and application of the new generation of catalysts.
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1 retracted
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A metal-free bifunctional electrocatalyst for oxygen reduction and oxygen evolution reactions
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Self-citationPhotochemical route for synthesizing atomically dispersed palladium catalysts
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Cited by
2D graphdiyne: An emerging carbon material
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Self-citationSingle Carbon Vacancy Traps Atomic Platinum for Hydrogen Evolution Catalysis
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Green ammonia production technologies: A review of practical progress
Ojelade, O. A., Zaman, S. F., & Ni, B.-J. (2023) · Journal of Environmental Management · doi:10.1016/j.jenvman.2023.118348 · Cited by 172
Dual-atom Co-Fe catalysts for oxygen reduction reaction
Tang, T., Wang, Y., Han, J., Zhang, Q., Bai, X., Niu, X., Wang, Z., & Guan, J. (2023) · Chinese Journal of Catalysis · doi:10.1016/s1872-2067(22)64189-5 · Cited by 113
Yu, J., Li, Z., Liu, T., Zhao, S., Guan, D., Chen, D., Shao, Z., & Ni, M. (2023) · Chemical Engineering Journal · doi:10.1016/j.cej.2023.141674 · Cited by 99
Metadata
- Authors
- Hui, L., Xue, Y., Yu, H., Liu, Y., Fang, Y., Xing, C., Huang, B., & Li, Y.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-05-31
- Volume
- 141
- Issue
- 27
- Pages
- 10677-10683
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2947393453
- Cited by
- 587
- References
- 46
- FWCI
- 18.77
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hui, L., Xue, Y., Yu, H., Liu, Y., Fang, Y., Xing, C., Huang, B., & Li, Y. (2019). Highly Efficient and Selective Generation of Ammonia and Hydrogen on a Graphdiyne-Based Catalyst. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.9b03004
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