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One-Dimensional Optoelectronic Nanostructures Derived from the Aqueous Self-Assembly of π-Conjugated Oligopeptides
Abstract
The aqueous self-assembly of oligopeptide-flanked pi-conjugated molecules into discrete one-dimensional nanostructures is described. Unique to these molecules is the fact that the pi-conjugated unit has been directly embedded within the peptide backbone by way of a synthetic amino acid with pi-functionality that is compatible with standard Fmoc-based peptide synthesis. The peptide-based molecular design enforces intimate pi-pi communication within the aggregate after charge-screening and self-assembly, making these nanostructures attractive for optical or electronic applications in biological environments. The synthesis and assembly are reported along with spectroscopic and morphological characterization of the new nanomaterials.
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Citations
Cited by
Functional π-Gelators and Their Applications
Babu, S. S., Praveen, V. K., & Ajayaghosh, A. (2014) · Chemical Reviews · doi:10.1021/cr400195e · Cited by 1,725
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Piepenbrock, M.-O. M., Lloyd, G. O., Clarke, N., & Steed, J. W. (2010) · Chemical Reviews · doi:10.1021/cr9003067 · Cited by 1,199
Investigating the optimal size of anticancer nanomedicine
Tang, L., Yang, X., Yin, Q., Cai, K., Wang, H., Chaudhury, I., Yao, C., Zhou, Q., Kwon, M., Hartman, J. A., et al. (2014) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1411499111 · Cited by 654
Peptide-Based Supramolecular Systems Chemistry
Sheehan, F., Sementa, D., Jain, A., Kumar, M., Tayarani-Najjaran, M., Kroiss, D., & Ulijn, R. V. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00089 · Cited by 428
Prebiotic Peptides: Molecular Hubs in the Origin of Life
Frenkel-Pinter, M., Samanta, M., Ashkenasy, G., & Leman, L. J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00664 · Cited by 354
Metadata
- Authors
- Diegelmann, S. R., Gorham, J. M., & Tovar, J. D.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-09-25
- Volume
- 130
- Issue
- 42
- Pages
- 13840-13841
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2027659235
- Cited by
- 162
- References
- 0
- FWCI
- 5.18
- Type
- journal article
- Language
- en
- Open access
- closed
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- Diegelmann, S. R., Gorham, J. M., & Tovar, J. D. (2008). One-Dimensional Optoelectronic Nanostructures Derived from the Aqueous Self-Assembly of π-Conjugated Oligopeptides. Journal of the American Chemical Society. https://doi.org/10.1021/ja805491d
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