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Layer-by-Layer Assembly of All Carbon Nanotube Ultrathin Films for Electrochemical Applications
Abstract
All multiwall carbon nanotube (MWNT) thin films are created by layer-by-layer (LBL) assembly of surface functionalized MWNTs. Negatively and positively charged MWNTs were prepared by surface functionalization, allowing the incorporation of MWNTs into highly tunable thin films via the LBL technique. The pH dependent surface charge on the MWNTs gives this system the unique characteristics of LBL assembly of weak polyelectrolytes, controlling thickness and morphology with assembly pH conditions. We demonstrate that these MWNT thin films have randomly oriented interpenetrating network structure with well developed nanopores using AFM and SEM, which is an ideal structure of functional materials for various applications. In particular, electrochemical measurements of these all-MWNT thin film electrodes show high electronic conductivity in comparison with polymer composites with single wall nanotubes, and high capacitive behavior with precise control of capacity.
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Cites
Noncovalent sidewall functionalization of single-walled carbon nanotubes for protein immobilization
Chen, R. J., Zhang, Y., Wang, D., & Dai, H. (2001) · Journal of the American Chemical Society · doi:10.1021/ja010172b · Cited by 2,534
Cited by
Georgakilas, V., Perman, J. A., Tucek, J., & Zboril, R. (2015) · Chemical Reviews · doi:10.1021/cr500304f · Cited by 2,147
Nanoporous metal/oxide hybrid electrodes for electrochemical supercapacitors
Lang, X., Hirata, A., Fujita, T., & Chen, M. (2011) · Nature Nanotechnology · doi:10.1038/nnano.2011.13 · Cited by 2,109
Wang, Q., Yan, J., & Fan, Z. (2016) · Energy & Environmental Science · doi:10.1039/c5ee03109e · Cited by 1,225
Electrocatalytic Oxygen Evolution at Surface-Oxidized Multiwall Carbon Nanotubes
Lu, X., Yim, W.-L., Suryanto, B. H. R., & Zhao, C. (2015) · Journal of the American Chemical Society · doi:10.1021/ja509879r · Cited by 594
On the Configuration of Supercapacitors for Maximizing Electrochemical Performance
Zhang, J., & Zhao, X. S. (2012) · ChemSusChem · doi:10.1002/cssc.201100571 · Cited by 527
Metadata
- Authors
- Lee, S. W., Kim, B.-S., Chen, S., Shao-Horn, Y., & Hammond, P. T.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-12-23
- Volume
- 131
- Issue
- 2
- Pages
- 671-679
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2064394331
- Cited by
- 648
- References
- 1
- FWCI
- 21.73
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lee, S. W., Kim, B.-S., Chen, S., Shao-Horn, Y., & Hammond, P. T. (2009). Layer-by-Layer Assembly of All Carbon Nanotube Ultrathin Films for Electrochemical Applications. Journal of the American Chemical Society. https://doi.org/10.1021/ja807059k
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
